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Atmospheric Measurement Techniques An interactive open-access journal of the European Geosciences Union

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Atmos. Meas. Tech., 7, 3783-3799, 2014
© Author(s) 2014. This work is distributed
under the Creative Commons Attribution 3.0 License.
Research article
18 Nov 2014
Validation of nine years of MOPITT V5 NIR using MOZAIC/IAGOS measurements: biases and long-term stability
A. T. J. de Laat1, I. Aben2, M. Deeter3, P. Nédélec4, H. Eskes1, J.-L. Attié4,5, P. Ricaud5, R. Abida5, L. El Amraoui5, and J. Landgraf2 1Royal Netherlands Meteorological Institute, de Bilt, the Netherlands
2Netherlands Space Research Institute, Utrecht, the Netherlands
3National Center for Atmospheric Research, Boulder, USA
4Laboratoire d'Aérologie-OMP, Université de Toulouse – CNRS/INSU, UMR5560, Toulouse, France
5CNRM-GAME Météo-France/CNRS UMR 3589, Toulouse, France
Abstract. Validation results from a comparison between Measurement Of Pollution In The Troposphere (MOPITT) V5 Near InfraRed (NIR) carbon monoxide (CO) total column measurements and Measurement of Ozone and Water Vapour on Airbus in-service Aircraft (MOZAIC)/In-Service Aircraft for a Global Observing System (IAGOS) aircraft measurements are presented. A good agreement is found between MOPITT and MOZAIC/IAGOS measurements, consistent with results from earlier studies using different validation data and despite large variability in MOPITT CO total columns along the spatial footprint of the MOZAIC/IAGOS measurements. Validation results improve when taking the large spatial footprint of the MOZAIC/IAGOS data into account. No statistically significant drift was detected in the validation results over the period 2002–2010 at global, continental and local (airport) scales. Furthermore, for those situations where MOZAIC/IAGOS measurements differed from the MOPITT a priori, the MOPITT measurements clearly outperformed the MOPITT a priori data, indicating that MOPITT NIR retrievals add value to the MOPITT a priori. Results from a high spatial resolution simulation of the chemistry-transport model MOCAGE (MOdèle de Chimie Atmosphérique à Grande Echelle) showed that the most likely explanation for the large MOPITT variability along the MOZAIC-IAGOS profile flight path is related to spatio-temporal CO variability, which should be kept in mind when using MOZAIC/IAGOS profile measurements for validating satellite nadir observations.

Citation: de Laat, A. T. J., Aben, I., Deeter, M., Nédélec, P., Eskes, H., Attié, J.-L., Ricaud, P., Abida, R., El Amraoui, L., and Landgraf, J.: Validation of nine years of MOPITT V5 NIR using MOZAIC/IAGOS measurements: biases and long-term stability, Atmos. Meas. Tech., 7, 3783-3799, doi:10.5194/amt-7-3783-2014, 2014.
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