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Atmospheric Measurement Techniques An interactive open-access journal of the European Geosciences Union

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Atmos. Meas. Tech., 10, 119-153, 2017
https://doi.org/10.5194/amt-10-119-2017
© Author(s) 2017. This work is distributed under
the Creative Commons Attribution 3.0 License.
Research article
09 Jan 2017
Sulfur dioxide retrievals from TROPOMI onboard Sentinel-5 Precursor: algorithm theoretical basis
Nicolas Theys1, Isabelle De Smedt1, Huan Yu1, Thomas Danckaert1, Jeroen van Gent1, Christoph Hörmann2, Thomas Wagner2, Pascal Hedelt3, Heiko Bauer3, Fabian Romahn3, Mattia Pedergnana3, Diego Loyola3, and Michel Van Roozendael1 1Royal Belgian Institute for Space Aeronomy (BIRA-IASB), Brussels, Belgium
2Max Planck Institute for Chemistry (MPIC), Hahn-Meitner-Weg 1, 55128 Mainz, Germany
3Institut für Methodik der Fernerkundung (IMF), Deutsches Zentrum für Luft und Raumfahrt (DLR), Oberpfaffenhofen, Germany
Abstract. The TROPOspheric Monitoring Instrument (TROPOMI) onboard the Copernicus Sentinel-5 Precursor (S-5P) platform will measure ultraviolet earthshine radiances at high spectral and improved spatial resolution (pixel size of 7 km  ×  3.5 km at nadir) compared to its predecessors OMI and GOME-2. This paper presents the sulfur dioxide (SO2) vertical column retrieval algorithm implemented in the S-5P operational processor UPAS (Universal Processor for UV/VIS Atmospheric Spectrometers) and comprehensively describes its various retrieval steps. The spectral fitting is performed using the differential optical absorption spectroscopy (DOAS) method including multiple fitting windows to cope with the large range of atmospheric SO2 columns encountered. It is followed by a slant column background correction scheme to reduce possible biases or across-track-dependent artifacts in the data. The SO2 vertical columns are obtained by applying air mass factors (AMFs) calculated for a set of representative a priori profiles and accounting for various parameters influencing the retrieval sensitivity to SO2. Finally, the algorithm includes an error analysis module which is fully described here. We also discuss verification results (as part of the algorithm development) and future validation needs of the TROPOMI SO2 algorithm.

Citation: Theys, N., De Smedt, I., Yu, H., Danckaert, T., van Gent, J., Hörmann, C., Wagner, T., Hedelt, P., Bauer, H., Romahn, F., Pedergnana, M., Loyola, D., and Van Roozendael, M.: Sulfur dioxide retrievals from TROPOMI onboard Sentinel-5 Precursor: algorithm theoretical basis, Atmos. Meas. Tech., 10, 119-153, https://doi.org/10.5194/amt-10-119-2017, 2017.
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Short summary
This paper provides a thorough description of the algorithm to retrieve SO2 columns from TROPOMI/Sentinel-5 Precursor measurements. The different algorithmic steps including error analysis are detailed. Scientific verification of the algorithm and validation needs are also discussed.
This paper provides a thorough description of the algorithm to retrieve SO2 columns from...
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