Articles | Volume 11, issue 5
https://doi.org/10.5194/amt-11-2653-2018
© Author(s) 2018. This work is distributed under
the Creative Commons Attribution 4.0 License.
the Creative Commons Attribution 4.0 License.
https://doi.org/10.5194/amt-11-2653-2018
© Author(s) 2018. This work is distributed under
the Creative Commons Attribution 4.0 License.
the Creative Commons Attribution 4.0 License.
Research article
| 
07 May 2018
Research article |
| 07 May 2018
| 07 May 2018
How well can global chemistry models calculate the reactivity of short-lived greenhouse gases in the remote troposphere, knowing the chemical composition
Department of Earth System Science, University of California, Irvine,
CA 92697-3100, USA
Clare M. Flynn
Department of Earth System Science, University of California, Irvine,
CA 92697-3100, USA
Xin Zhu
Department of Earth System Science, University of California, Irvine,
CA 92697-3100, USA
Stephen D. Steenrod
NASA Goddard Space Flight Center, Greenbelt, MD, USA
Universities Space Research Association (USRA), GESTAR, Columbia, MD,
USA
Sarah A. Strode
NASA Goddard Space Flight Center, Greenbelt, MD, USA
Universities Space Research Association (USRA), GESTAR, Columbia, MD,
USA
Arlene M. Fiore
Department of Earth and Environmental Sciences and Lamont-Doherty
Earth Observatory of Columbia University, Palisades, NY, USA
Gustavo Correa
Department of Earth and Environmental Sciences and Lamont-Doherty
Earth Observatory of Columbia University, Palisades, NY, USA
Lee T. Murray
Department of Earth and Environmental Sciences, University of
Rochester, Rochester, NY 14627-0221, USA
Jean-Francois Lamarque
Atmospheric Chemistry, Observations and Modeling Laboratory, National
Center for Atmospheric Research, Boulder, CO 80301, USA
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Cited
11 citations as recorded by crossref.
- Heterogeneity and chemical reactivity of the remote troposphere defined by aircraft measurements H. Guo et al. 10.5194/acp-21-13729-2021
- Forecasting carbon monoxide on a global scale for the ATom-1 aircraft mission: insights from airborne and satellite observations and modeling S. Strode et al. 10.5194/acp-18-10955-2018
- Deconstruction of tropospheric chemical reactivity using aircraft measurements: the Atmospheric Tomography Mission (ATom) data M. Prather et al. 10.5194/essd-15-3299-2023
- Cloud impacts on photochemistry: building a climatology of photolysis rates from the Atmospheric Tomography mission S. Hall et al. 10.5194/acp-18-16809-2018
- Mapping hydroxyl variability throughout the global remote troposphere via synthesis of airborne and satellite formaldehyde observations G. Wolfe et al. 10.1073/pnas.1821661116
- Radiative Forcing of Climate: The Historical Evolution of the Radiative Forcing Concept, the Forcing Agents and their Quantification, and Applications V. Ramaswamy et al. 10.1175/AMSMONOGRAPHS-D-19-0001.1
- H2O2 and CH3OOH (MHP) in the Remote Atmosphere: 1. Global Distribution and Regional Influences H. Allen et al. 10.1029/2021JD035701
- An observation-based, reduced-form model for oxidation in the remote marine troposphere C. Baublitz et al. 10.1073/pnas.2209735120
- Heterogeneity and chemical reactivity of the remote troposphere defined by aircraft measurements – corrected H. Guo et al. 10.5194/acp-23-99-2023
- Investigation of fuel consumption of a passenger car depending on aerodynamic resistance and related aspects: a case study O. Stopka et al. 10.14669/AM.VOL81.ART9
- Change in Tropospheric Ozone in the Recent Decades and Its Contribution to Global Total Ozone J. Liu et al. 10.1029/2022JD037170
11 citations as recorded by crossref.
- Heterogeneity and chemical reactivity of the remote troposphere defined by aircraft measurements H. Guo et al. 10.5194/acp-21-13729-2021
- Forecasting carbon monoxide on a global scale for the ATom-1 aircraft mission: insights from airborne and satellite observations and modeling S. Strode et al. 10.5194/acp-18-10955-2018
- Deconstruction of tropospheric chemical reactivity using aircraft measurements: the Atmospheric Tomography Mission (ATom) data M. Prather et al. 10.5194/essd-15-3299-2023
- Cloud impacts on photochemistry: building a climatology of photolysis rates from the Atmospheric Tomography mission S. Hall et al. 10.5194/acp-18-16809-2018
- Mapping hydroxyl variability throughout the global remote troposphere via synthesis of airborne and satellite formaldehyde observations G. Wolfe et al. 10.1073/pnas.1821661116
- Radiative Forcing of Climate: The Historical Evolution of the Radiative Forcing Concept, the Forcing Agents and their Quantification, and Applications V. Ramaswamy et al. 10.1175/AMSMONOGRAPHS-D-19-0001.1
- H2O2 and CH3OOH (MHP) in the Remote Atmosphere: 1. Global Distribution and Regional Influences H. Allen et al. 10.1029/2021JD035701
- An observation-based, reduced-form model for oxidation in the remote marine troposphere C. Baublitz et al. 10.1073/pnas.2209735120
- Heterogeneity and chemical reactivity of the remote troposphere defined by aircraft measurements – corrected H. Guo et al. 10.5194/acp-23-99-2023
- Investigation of fuel consumption of a passenger car depending on aerodynamic resistance and related aspects: a case study O. Stopka et al. 10.14669/AM.VOL81.ART9
- Change in Tropospheric Ozone in the Recent Decades and Its Contribution to Global Total Ozone J. Liu et al. 10.1029/2022JD037170
Latest update: 16 Apr 2024
Short summary
A new protocol for merging in situ atmospheric chemistry measurements with 3-D models is developed. This technique can identify the most reactive air parcels in terms of tropospheric production/loss of O3 & CH4. This approach highlights differences in 6 global chemistry models even with composition specified. Thus in situ measurements from, e.g., NASA's ATom mission can be used to develop a chemical climatology of, not only the key species, but also the rates of key reactions in each air parcel.
A new protocol for merging in situ atmospheric chemistry measurements with 3-D models is...
