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AMT | Articles | Volume 11, issue 7
Atmos. Meas. Tech., 11, 4345–4360, 2018
https://doi.org/10.5194/amt-11-4345-2018
© Author(s) 2018. This work is distributed under
the Creative Commons Attribution 4.0 License.
Atmos. Meas. Tech., 11, 4345–4360, 2018
https://doi.org/10.5194/amt-11-4345-2018
© Author(s) 2018. This work is distributed under
the Creative Commons Attribution 4.0 License.

Research article 23 Jul 2018

Research article | 23 Jul 2018

Exploring femtosecond laser ablation in single-particle aerosol mass spectrometry

Ramakrishna Ramisetty et al.
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Cited articles  
Amoruso, S., Bruzzese, R., Spinelli, N., and Velotta, R.: Characterization of laser-ablation plasmas, J. Phys. B-At. Mol. Opt., 32, R131, https://doi.org/10.1088/0953-4075/32/14/201, 1999. 
Bhave, P. V., Allen, J. O., Morrical, B. D., Fergenson, D. P., Cass, G. R., and Prather, K. A.: A Field-Based Approach for Determining ATOFMS Instrument Sensitivities to Ammonium and Nitrate, Environ. Sci. Technol., 36, 4868–4879, 2001. 
Brands, M., Kamphus, M., Böttger, T., Schneider, J., Drewnick, F., Roth, A., Curtius, J., Voigt, C., Borbon, A., Beekmann, M., Bourdon, A., Perrin, T., and Borrmann, S.: Characterization of a Newly Developed Aircraft-Based Laser Ablation Aerosol Mass Spectrometer (ALABAMA) and First Field Deployment in Urban Pollution Plumes over Paris During MEGAPOLI 2009, Aerosol Sci. Tech., 45, 46–64, 2011. 
Bulgakov, A. V., Ozerov, I., and Marine, W.: Silicon clusters produced by femtosecond laser ablation: non-thermal emission and gas-phase condensation, Appl. Phys. A, 79, 1591–1594, 2004. 
Cabalo, J., Zelenyuk, A., Baer, T., and Miller, R. E.: Two-Color Laser Induced Evaporation Dynamics of Liquid Aerosols Probed by Time-of-Flight Mass Spectrometry, Aerosol Sci. Tech., 33, 3-19, 2000. 
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Short summary
In this study we coupled a laser ablation aerosol time-of-flight (LAAPTOF) single-particle mass spectrometer, originally equipped with an excimer laser, to a femtosecond laser. The objective was to assess the influence of the higher laser power density of the femtosecond laser on ablation–ionization of atmospheric particles, ion signal, and ultimately quantitative abilities of the single-particle mass spectrometer.
In this study we coupled a laser ablation aerosol time-of-flight (LAAPTOF) single-particle mass...
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