Articles | Volume 11, issue 9
https://doi.org/10.5194/amt-11-5299-2018
© Author(s) 2018. This work is distributed under
the Creative Commons Attribution 4.0 License.
the Creative Commons Attribution 4.0 License.
https://doi.org/10.5194/amt-11-5299-2018
© Author(s) 2018. This work is distributed under
the Creative Commons Attribution 4.0 License.
the Creative Commons Attribution 4.0 License.
Research article
| 
20 Sep 2018
Research article |
| 20 Sep 2018
| 20 Sep 2018
Photocurrent modelling and experimental confirmation for meteoric smoke particle detectors on board atmospheric sounding rockets
Gabriel Giono
CORRESPONDING AUTHOR
Leibniz Institute of Atmospheric Physics at the Rostock University
(IAP), Kühlungsborn, Germany
Department of Space and Plasma
Physics, School of Electrical Engineering, KTH-Royal Institute of
Technology, Stockholm, Sweden
Boris Strelnikov
Leibniz Institute of Atmospheric Physics at the Rostock University
(IAP), Kühlungsborn, Germany
Heiner Asmus
Leibniz Institute of Atmospheric Physics at the Rostock University
(IAP), Kühlungsborn, Germany
Tristan Staszak
Leibniz Institute of Atmospheric Physics at the Rostock University
(IAP), Kühlungsborn, Germany
Nickolay Ivchenko
Department of Space and Plasma
Physics, School of Electrical Engineering, KTH-Royal Institute of
Technology, Stockholm, Sweden
Franz-Josef Lübken
Leibniz Institute of Atmospheric Physics at the Rostock University
(IAP), Kühlungsborn, Germany
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Minna Palmroth, Maxime Grandin, Theodoros Sarris, Eelco Doornbos, Stelios Tourgaidis, Anita Aikio, Stephan Buchert, Mark A. Clilverd, Iannis Dandouras, Roderick Heelis, Alex Hoffmann, Nickolay Ivchenko, Guram Kervalishvili, David J. Knudsen, Anna Kotova, Han-Li Liu, David M. Malaspina, Günther March, Aurélie Marchaudon, Octav Marghitu, Tomoko Matsuo, Wojciech J. Miloch, Therese Moretto-Jørgensen, Dimitris Mpaloukidis, Nils Olsen, Konstantinos Papadakis, Robert Pfaff, Panagiotis Pirnaris, Christian Siemes, Claudia Stolle, Jonas Suni, Jose van den IJssel, Pekka T. Verronen, Pieter Visser, and Masatoshi Yamauchi
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Atmos. Meas. Tech., 12, 4191–4210, https://doi.org/10.5194/amt-12-4191-2019, https://doi.org/10.5194/amt-12-4191-2019, 2019
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Jacob Zalach, Christian von Savigny, Arvid Langenbach, Gerd Baumgarten, Franz-Josef Lübken, and Adam Bourassa
Atmos. Meas. Tech. Discuss., https://doi.org/10.5194/amt-2019-267, https://doi.org/10.5194/amt-2019-267, 2019
Revised manuscript not accepted
Arvid Langenbach, Gerd Baumgarten, Jens Fiedler, Franz-Josef Lübken, Christian von Savigny, and Jacob Zalach
Atmos. Meas. Tech., 12, 4065–4076, https://doi.org/10.5194/amt-12-4065-2019, https://doi.org/10.5194/amt-12-4065-2019, 2019
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Stratospheric aerosol backscatter ratios in the Arctic using Rayleigh, Mie and Raman backscattered signals were calculated. A backscatter ratio calculation during daytime was performed for the first time. Sharp aerosol layers thinner than 1 km over several days were observed. The seasonal cycle of stratospheric background aerosol in high latitudes including the summer months was calculated for the first time. Top altitude of the aerosol layer was found to reach up to 34 km, especially in summer.
Martin Eberhart, Stefan Löhle, Boris Strelnikov, Jonas Hedin, Mikhail Khaplanov, Stefanos Fasoulas, Jörg Gumbel, Franz-Josef Lübken, and Markus Rapp
Atmos. Meas. Tech., 12, 2445–2461, https://doi.org/10.5194/amt-12-2445-2019, https://doi.org/10.5194/amt-12-2445-2019, 2019
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This paper describes the measurement of atomic oxygen in the upper atmosphere onboard sounding rockets using solid electrolyte sensors. Calibration of the sensors in the laboratory is explained in detail. Results from the WADIS-2 rocket campaign show profiles of atomic oxygen density with a high spatial resolution.
Uwe Berger, Gerd Baumgarten, Jens Fiedler, and Franz-Josef Lübken
Atmos. Chem. Phys., 19, 4685–4702, https://doi.org/10.5194/acp-19-4685-2019, https://doi.org/10.5194/acp-19-4685-2019, 2019
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In this paper we present a new description of statistical probability density functions (pdfs) of polar mesospheric clouds (PMC). We derive a new class of pdfs that describes successfully the probability statistic of ALOMAR lidar observations of different ice parameters. As a main advantage the new method allows us to connect different observational PMC distributions of lidar and satellite data, and also to compare with distributions from ice model studies.
Mykhaylo Grygalashvyly, Martin Eberhart, Jonas Hedin, Boris Strelnikov, Franz-Josef Lübken, Markus Rapp, Stefan Löhle, Stefanos Fasoulas, Mikhail Khaplanov, Jörg Gumbel, and Ekaterina Vorobeva
Atmos. Chem. Phys., 19, 1207–1220, https://doi.org/10.5194/acp-19-1207-2019, https://doi.org/10.5194/acp-19-1207-2019, 2019
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Based on rocket-borne true common volume observations of atomic oxygen, atmospheric band emission (762 nm), and background atmosphere density and temperature, one-step, two-step, and combined mechanisms of
O2(b1Σg+) formation were analyzed. We found new coefficients for the fit function based on self-consistent temperature, atomic oxygen, and volume emission observations. This can be used for atmospheric band volume emission modeling or the estimation of atomic oxygen by known volume emission.
Raimund Wörl, Boris Strelnikov, Timo P. Viehl, Josef Höffner, Pierre-Dominique Pautet, Michael J. Taylor, Yucheng Zhao, and Franz-Josef Lübken
Atmos. Chem. Phys., 19, 77–88, https://doi.org/10.5194/acp-19-77-2019, https://doi.org/10.5194/acp-19-77-2019, 2019
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Simultaneous temperature measurements during the WADIS-2 rocket campaign are used to investigate the thermal structure of the mesopause region. Vertically and horizontally resolved in situ and remote measurements are in good agreement and show dominating long-term and large-scale waves with periods of 24 h and higher tidal harmonics. Only a few gravity waves with periods shorter than 6 h and small amplitudes are there.
Michael Gerding, Jochen Zöllner, Marius Zecha, Kathrin Baumgarten, Josef Höffner, Gunter Stober, and Franz-Josef Lübken
Atmos. Chem. Phys., 18, 15569–15580, https://doi.org/10.5194/acp-18-15569-2018, https://doi.org/10.5194/acp-18-15569-2018, 2018
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We describe the first comparative study of noctilucent clouds (NLCs) and mesospheric summer echoes at midlatitudes. Therefore, this study compares fresh clouds (small particles) with fully evolved clouds in the mesosphere, hinting at their evolution. It is shown that, in contrast to higher latitudes, here only a thin layer of fresh particles exist above the NLCs. This gives evidence that NLCs are not formed locally but are typically advected. This needs to be acknowledged in trend studies.
Gerald A. Lehmacher, Miguel F. Larsen, Richard L. Collins, Aroh Barjatya, and Boris Strelnikov
Ann. Geophys., 36, 1099–1116, https://doi.org/10.5194/angeo-36-1099-2018, https://doi.org/10.5194/angeo-36-1099-2018, 2018
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We used sounding rockets to obtain four high-resolution temperature profiles in the mesosphere over a limited area. We found consistent deep isothermal and adiabatic layers, but variable and finely structured turbulence preferentially in the lower stable mesosphere. Accompanying tracer releases showed horizontal winds in the lower thermosphere with extreme shears and 200 m s−1 winds under moderately disturbed geomagnetic conditions, and convection-like structures just below the mesopause.
Francie Schmidt, Gerd Baumgarten, Uwe Berger, Jens Fiedler, and Franz-Josef Lübken
Atmos. Chem. Phys., 18, 8893–8908, https://doi.org/10.5194/acp-18-8893-2018, https://doi.org/10.5194/acp-18-8893-2018, 2018
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Local time variations of polar mesospheric clouds (PMCs) in the Northern Hemisphere are studied using a combination of a global circulation model and a microphysical model. We investigate the brightness, altitude, and occurrence of the clouds and find a good agreement between model and observations. The variations are caused by tidal structures in background parameters. The temperature varies by about 2 K and water vapor by about 3 ppmv at the altitude of ice particle sublimation near 81.5 km.
Rolf Rüfenacht, Gerd Baumgarten, Jens Hildebrand, Franziska Schranz, Vivien Matthias, Gunter Stober, Franz-Josef Lübken, and Niklaus Kämpfer
Atmos. Meas. Tech., 11, 1971–1987, https://doi.org/10.5194/amt-11-1971-2018, https://doi.org/10.5194/amt-11-1971-2018, 2018
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Wind information throughout the middle-atmosphere is crucial for the understanding of atmospheric dynamics but became available only recently, thanks to developments in remote sensing and modelling approaches. We present the first thorough assessment of the quality of the wind estimates by comparing co-located observations from lidar and microwave radiometry and opposing them to the major atmospheric models. Moreover we evaluated a new approach for measuring mesopause region wind by radiometry.
Kathrin Baumgarten, Michael Gerding, Gerd Baumgarten, and Franz-Josef Lübken
Atmos. Chem. Phys., 18, 371–384, https://doi.org/10.5194/acp-18-371-2018, https://doi.org/10.5194/acp-18-371-2018, 2018
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Gravity waves (GWs) as well as solar tides are a key driving mechanism for the circulation in the Earth's atmosphere. The temporal variation of these waves is studied using a record long 10-day continuous Rayleigh–Mie–Raman lidar sounding at midlatitudes. This data set shows a large variability of these waves on timescales of a few days and therefore provides new insights into wave intermittency phenomena, which can help to improve model simulations.
Jens Hildebrand, Gerd Baumgarten, Jens Fiedler, and Franz-Josef Lübken
Atmos. Chem. Phys., 17, 13345–13359, https://doi.org/10.5194/acp-17-13345-2017, https://doi.org/10.5194/acp-17-13345-2017, 2017
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We present altitude profiles of winds and temperatures in the Arctic strato- and mesosphere obtained during three Januaries. The data show large year-to-year variations. We compare the observations to model data. For monthly mean profiles we find good agreement below 55 km altitude but also differences of up to 20 K and 20 m s-1 above. The fluctuations during single nights indicate gravity waves. The kinetic energy of such waves is typically 5 to 10 times larger than their potential energy.
Nickolay Ivchenko, Nicola M. Schlatter, Hanna Dahlgren, Yasunobu Ogawa, Yuka Sato, and Ingemar Häggström
Ann. Geophys., 35, 1143–1149, https://doi.org/10.5194/angeo-35-1143-2017, https://doi.org/10.5194/angeo-35-1143-2017, 2017
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Photo-electrons and secondary electrons from particle precipitation enhance the incoherent scatter plasma line to levels sufficient for detection. A plasma line gives an accurate measure of the electron density and can be used to estimate electron temperature. The occurrence of plasma line enhancements in the EISCAT Svalbard Radar data was investigated. During summer daytime hours the plasma line is detectable in up to 90 % of the data. In winter time the occurrence is a few percent.
Heiner Asmus, Tristan Staszak, Boris Strelnikov, Franz-Josef Lübken, Martin Friedrich, and Markus Rapp
Ann. Geophys., 35, 979–998, https://doi.org/10.5194/angeo-35-979-2017, https://doi.org/10.5194/angeo-35-979-2017, 2017
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This work sheds new light on the size distribution of dust grains of meteoric origin in the mesosphere and lower thermosphere region using rocket-borne instrumentation. We found that a large number of very small (~ 0.5 nm) particles are charged and therefore have a significant influence on the charge balance of the lower ionosphere.
Andreas Schneider, Johannes Wagner, Jens Faber, Michael Gerding, and Franz-Josef Lübken
Atmos. Chem. Phys., 17, 7941–7954, https://doi.org/10.5194/acp-17-7941-2017, https://doi.org/10.5194/acp-17-7941-2017, 2017
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Wave breaking is studied with a combination of high-resolution turbulence observations with the balloon-borne instrument LITOS and mesoscale simulations with the WRF model. A relation between observed turbulent energy dissipation rates and the occurrence of wave patterns in modelled vertical winds is found, which is interpreted as the effect of wave saturation. The change of stability plays less of a role for mean dissipation for the flights examined.
Yunxia Yuan, Nickolay Ivchenko, Gunnar Tibert, Marin Stanev, Jonas Hedin, and Jörg Gumbel
Atmos. Meas. Tech. Discuss., https://doi.org/10.5194/amt-2017-91, https://doi.org/10.5194/amt-2017-91, 2017
Revised manuscript has not been submitted
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The paper presents a method to determine altitude profile of atmospheric density, temperature and wind by means of analysing the reconstructed trajectory of a rigid falling sphere released from a sounding rocket. The trajectory reconstruction is achieved by post-flight analysis of GPS raw data gathered in the sphere. A comparison of the results with independent measurements is presented, with good agreement of the falling sphere results with other sources in the stratosphere.
Boris Strelnikov, Artur Szewczyk, Irina Strelnikova, Ralph Latteck, Gerd Baumgarten, Franz-Josef Lübken, Markus Rapp, Stefanos Fasoulas, Stefan Löhle, Martin Eberhart, Ulf-Peter Hoppe, Tim Dunker, Martin Friedrich, Jonas Hedin, Mikhail Khaplanov, Jörg Gumbel, and Aroh Barjatya
Ann. Geophys., 35, 547–565, https://doi.org/10.5194/angeo-35-547-2017, https://doi.org/10.5194/angeo-35-547-2017, 2017
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The WADIS sounding rocket mission utilized multi-point turbulence measurements in the mesosphere by different techniques, i.e., with ionization gauges carried by rockets and ground-based MAARSY and EISCAT radars. Results show that turbulence energy dissipation rates oscillate in space and time with amplitude of up to 2 orders of magnitude. Spatial oscillations show the same wavelengths as atmospheric gravity waves. Temporal variability reveals periods of atmospheric tides and gravity waves.
Hanna Dahlgren, Betty S. Lanchester, Nickolay Ivchenko, and Daniel K. Whiter
Ann. Geophys., 35, 493–503, https://doi.org/10.5194/angeo-35-493-2017, https://doi.org/10.5194/angeo-35-493-2017, 2017
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Pulsating aurora are ubiquitous events that constitute a large amount of energy transfer to the ionosphere. Still there are unsolved issues regarding their formation. Using high-resolution optical and radar data, we find that it is the flux of high-energy electrons that get reduced during the OFF period of the pulsations. We also report on dips in brightness at the transition between ON and OFF, and asymmetric rise and fall times, which may have implications for understanding the pulsations.
Hanna Dahlgren, Nicola M. Schlatter, Nickolay Ivchenko, Lorenz Roth, and Alexander Karlsson
Ann. Geophys., 35, 475–479, https://doi.org/10.5194/angeo-35-475-2017, https://doi.org/10.5194/angeo-35-475-2017, 2017
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Anomalous strong echoes with three frequency peaks are occasionally seen with incoherent scatter radars in the ionosphere near 200 km altitude at high latitudes. We investigate how they relate to electron precipitation, by finding the resulting peak electron density and the height of the peak, respectively. We find that occurrence rate increases with density and decreases with height, indicating a correlation between the echoes and precipitating electrons with high energy and energy flux.
Franz-Josef Lübken, Gerd Baumgarten, Jens Hildebrand, and Francis J. Schmidlin
Atmos. Meas. Tech., 9, 3911–3919, https://doi.org/10.5194/amt-9-3911-2016, https://doi.org/10.5194/amt-9-3911-2016, 2016
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Wind measurements in the middle atmosphere (MA) are crucial to our understanding of atmospheric processes. We have recently developed a new laser-based method to measure winds called DoRIS (Doppler Rayleigh Iodine Spectrometer) which is the only technique to monitor winds in the middle atmosphere quasi-continuously. We
compare our measurements with rocket-borne measurements and find excellent
agreement above 30 km. DoRIS can now be considered as a validated method to measure winds in the MA.
Michael Gerding, Maren Kopp, Josef Höffner, Kathrin Baumgarten, and Franz-Josef Lübken
Atmos. Meas. Tech., 9, 3707–3715, https://doi.org/10.5194/amt-9-3707-2016, https://doi.org/10.5194/amt-9-3707-2016, 2016
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Temperature soundings by lidar are an important tool for the understanding of the middle atmosphere, including gravity waves and tides. Though, mesospheric lidar soundings at daytime are rare. We describe a daylight-capable RMR lidar with optical bandwidths in the range of the Doppler broadened laser backscatter. We account for the systematic temperature error induced by the optical filter, and present examples of daylight-independent temperature sounding as well as tidal analysis.
J. Kiliani, G. Baumgarten, F.-J. Lübken, and U. Berger
Atmos. Chem. Phys., 15, 12897–12907, https://doi.org/10.5194/acp-15-12897-2015, https://doi.org/10.5194/acp-15-12897-2015, 2015
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For the first time the shape of noctilucent cloud particles is analyzed with a 3-D Lagrangian model. Three-color lidar measurements are compared directly to optical modeling of NLC simulations with non-spherical shapes: a mix of elongated and flattened cylindrical ice particles consistent with measurements. Comparison is best if flattened particles form a majority, with mean axis ratio around 2.8. NLCs from cylindrical particles are slightly brighter and consist of fewer but larger ice particle.
N. M. Schlatter, V. Belyey, B. Gustavsson, N. Ivchenko, D. Whiter, H. Dahlgren, S. Tuttle, and T. Grydeland
Ann. Geophys., 33, 837–844, https://doi.org/10.5194/angeo-33-837-2015, https://doi.org/10.5194/angeo-33-837-2015, 2015
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The high-latitude ionosphere is a dynamic region where particle precipitation leads to various phenomena including wave instability and turbulence. Anomalous echoes related to aurora are observed in ground-based radar observations of the ionosphere. These echoes indicate enhanced ion acoustic fluctuations. In this article, we show that the origin of the echo is located in or close to the region of particle precipitation and that the echo region itself is limited to hundreds of meters.
A. Schneider, M. Gerding, and F.-J. Lübken
Atmos. Chem. Phys., 15, 2159–2166, https://doi.org/10.5194/acp-15-2159-2015, https://doi.org/10.5194/acp-15-2159-2015, 2015
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Stratospheric turbulence is essential for the atmospheric energy budget. We compare in situ observations with our LITOS method based on spectral analysis of mm-scale wind fluctuations with the Thorpe method applied to standard radiosondes. Energy dissipations rates from both methods differ by up to 3 orders of magnitude. Nevertheless, mean values are in good agreement. We present case studies on both methods and examine the applicability of the Thorpe method for calculation of dissipation rates.
N. Kaifler, G. Baumgarten, J. Fiedler, and F.-J. Lübken
Atmos. Chem. Phys., 13, 11757–11768, https://doi.org/10.5194/acp-13-11757-2013, https://doi.org/10.5194/acp-13-11757-2013, 2013
N. M. Schlatter, N. Ivchenko, T. Sergienko, B. Gustavsson, and B. U. E. Brändström
Ann. Geophys., 31, 1681–1687, https://doi.org/10.5194/angeo-31-1681-2013, https://doi.org/10.5194/angeo-31-1681-2013, 2013
N. M. Schlatter, N. Ivchenko, B. Gustavsson, T. Leyser, and M. Rietveld
Ann. Geophys., 31, 1103–1108, https://doi.org/10.5194/angeo-31-1103-2013, https://doi.org/10.5194/angeo-31-1103-2013, 2013
A. Szewczyk, B. Strelnikov, M. Rapp, I. Strelnikova, G. Baumgarten, N. Kaifler, T. Dunker, and U.-P. Hoppe
Ann. Geophys., 31, 775–785, https://doi.org/10.5194/angeo-31-775-2013, https://doi.org/10.5194/angeo-31-775-2013, 2013
W. Reid, P. Achtert, N. Ivchenko, P. Magnusson, T. Kuremyr, V. Shepenkov, and G. Tibert
Atmos. Meas. Tech., 6, 777–785, https://doi.org/10.5194/amt-6-777-2013, https://doi.org/10.5194/amt-6-777-2013, 2013
M. Rapp, J. M. C. Plane, B. Strelnikov, G. Stober, S. Ernst, J. Hedin, M. Friedrich, and U.-P. Hoppe
Ann. Geophys., 30, 1661–1673, https://doi.org/10.5194/angeo-30-1661-2012, https://doi.org/10.5194/angeo-30-1661-2012, 2012
Related subject area
Subject: Aerosols | Technique: In Situ Measurement | Topic: Instruments and Platforms
Modular Multiplatform Compatible Air Measurement System (MoMuCAMS): a new modular platform for boundary layer aerosol and trace gas vertical measurements in extreme environments
Two new multirotor uncrewed aerial vehicles (UAVs) for glaciogenic cloud seeding and aerosol measurements within the CLOUDLAB project
Real-time pollen identification using holographic imaging and fluorescence measurements
Assessing potential indicators of aerosol wet scavenging during long-range transport
Next-generation ice-nucleating particle sampling on board aircraft: characterization of the High-volume flow aERosol particle filter sAmpler (HERA)
Development of a cascade impactor optimised for size-fractionated analysis of aerosol metal content by total reflection X-ray fluorescence spectroscopy (TXRF)
Development and characterization of the Portable Ice Nucleation Chamber 2 (PINCii)
Large-scale automated emission measurement of individual vehicles with point sampling
The four-wavelength Photoacoustic Aerosol Absorption Spectrometer (PAAS-4λ)
Improved counting statistics of an ultrafine differential mobility particle size spectrometer system
Performance evaluation of the Alphasense OPC-N3 and Plantower PMS5003 sensor in measuring dust events in the Salt Lake Valley, Utah
Characterization of the airborne aerosol inlet and transport system used during the A-LIFE aircraft field experiment
Source apportionment of black carbon and combustion-related CO2 for the determination of source-specific emission factors
CAMP: an instrumented platform for balloon-borne aerosol particle studies in the lower atmosphere
New method to determine black carbon mass size distribution
The realization of autonomous, aircraft-based, real-time aerosol mass spectrometry in the upper troposphere and lower stratosphere
A study on the performance of low-cost sensors for source apportionment at an urban background site
A dual-wavelength photothermal aerosol absorption monitor: design, calibration and performance
A high-transmission axial ion mobility classifier for mass–mobility measurements of atmospheric ions
Design, characterization, and first field deployment of a novel aircraft-based aerosol mass spectrometer combining the laser ablation and flash vaporization techniques
An instrument for direct measurement of emissions: cooling tower example
The Aerosol Research Observation Station (AEROS)
Laser imaging nephelometer for aircraft deployment
A new method to quantify particulate sodium and potassium salts (nitrate, chloride, and sulfate) by thermal desorption aerosol mass spectrometry
Evaluating the PurpleAir monitor as an aerosol light scattering instrument
Undersizing of aged African biomass burning aerosol by an ultra-high-sensitivity aerosol spectrometer
Evaluation methods for low-cost particulate matter sensors
Simulation-aided characterization of a versatile water-based condensation particle counter for atmospheric airborne research
Development of an in situ dual-channel thermal desorption gas chromatography instrument for consistent quantification of volatile, intermediate-volatility and semivolatile organic compounds
Assessment of online water-soluble brown carbon measuring systems for aircraft sampling
Characterizing the performance of a POPS miniaturized optical particle counter when operated on a quadcopter drone
A low-cost monitor for simultaneous measurement of fine particulate matter and aerosol optical depth – Part 3: Automation and design improvements
Rapid measurement of RH-dependent aerosol hygroscopic growth using a humidity-controlled fast integrated mobility spectrometer (HFIMS)
Detection of ship plumes from residual fuel operation in emission control areas using single-particle mass spectrometry
Highly time-resolved characterization of carbonaceous aerosols using a two-wavelength Sunset thermal–optical carbon analyzer
Captive Aerosol Growth and Evolution (CAGE) chamber system to investigate particle growth due to secondary aerosol formation
Design and characterization of a new oxidation flow reactor for laboratory and long-term ambient studies
A reel-down instrument system for profile measurements of water vapor, temperature, clouds, and aerosol beneath constant-altitude scientific balloons
Airborne extractive electrospray mass spectrometry measurements of the chemical composition of organic aerosol
A semicontinuous study on the ecotoxicity of atmospheric particles using a versatile aerosol concentration enrichment system (VACES): development and field characterization
A novel rocket-borne ion mass spectrometer with large mass range: instrument description and first-flight results
Detailed characterization of the CAPS single-scattering albedo monitor (CAPS PMssa) as a field-deployable instrument for measuring aerosol light absorption with the extinction-minus-scattering method
New in situ aerosol hyperspectral optical measurements over 300–700 nm – Part 1: Spectral Aerosol Extinction (SpEx) instrument field validation during the KORUS-OC cruise
New in situ aerosol hyperspectral optical measurements over 300–700 nm – Part 2: Extinction, total absorption, water- and methanol-soluble absorption observed during the KORUS-OC cruise
Continuous online monitoring of ice-nucleating particles: development of the automated Horizontal Ice Nucleation Chamber (HINC-Auto)
Evaluation of optical particulate matter sensors under realistic conditions of strong and mild urban pollution
Optimizing the detection, ablation, and ion extraction efficiency of a single-particle laser ablation mass spectrometer for application in environments with low aerosol particle concentrations
Measurements of PM2.5 with PurpleAir under atmospheric conditions
Development and application of a mass closure PM2.5 composition online monitoring system
Improved chloride quantification in quadrupole aerosol chemical speciation monitors (Q-ACSMs)
Roman Pohorsky, Andrea Baccarini, Julie Tolu, Lenny H. E. Winkel, and Julia Schmale
Atmos. Meas. Tech., 17, 731–754, https://doi.org/10.5194/amt-17-731-2024, https://doi.org/10.5194/amt-17-731-2024, 2024
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This manuscript presents a new tethered-balloon-based platform for in situ vertical measurements of aerosols and trace gases in the lower atmosphere of polar and alpine regions. The system can host various instrumental setups to target different research questions and features new instruments, in particular a miniaturized scanning electrical mobility spectrometer, deployed for the first time in a tethered balloon.
Anna J. Miller, Fabiola Ramelli, Christopher Fuchs, Nadja Omanovic, Robert Spirig, Huiying Zhang, Ulrike Lohmann, Zamin A. Kanji, and Jan Henneberger
Atmos. Meas. Tech., 17, 601–625, https://doi.org/10.5194/amt-17-601-2024, https://doi.org/10.5194/amt-17-601-2024, 2024
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We present a method for aerosol and cloud research using two uncrewed aerial vehicles (UAVs). The UAVs have a propeller heating mechanism that allows flights in icing conditions, which has so far been a limitation for cloud research with UAVs. One UAV burns seeding flares, producing a plume of particles that causes ice formation in supercooled clouds. The second UAV measures aerosol size distributions and is used for measuring the seeding plume or for characterizing the boundary layer.
Sophie Erb, Elias Graf, Yanick Zeder, Simone Lionetti, Alexis Berne, Bernard Clot, Gian Lieberherr, Fiona Tummon, Pascal Wullschleger, and Benoît Crouzy
Atmos. Meas. Tech., 17, 441–451, https://doi.org/10.5194/amt-17-441-2024, https://doi.org/10.5194/amt-17-441-2024, 2024
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In this study, we focus on an automatic bioaerosol measurement instrument and investigate the impact of using its fluorescence measurement for pollen identification. The fluorescence signal is used together with a pair of images from the same instrument to identify single pollen grains via neural networks. We test whether considering fluorescence as a supplementary input improves the pollen identification performance by comparing three different neural networks.
Miguel Ricardo A. Hilario, Avelino F. Arellano, Ali Behrangi, Ewan C. Crosbie, Joshua P. DiGangi, Glenn S. Diskin, Michael A. Shook, Luke D. Ziemba, and Armin Sorooshian
Atmos. Meas. Tech., 17, 37–55, https://doi.org/10.5194/amt-17-37-2024, https://doi.org/10.5194/amt-17-37-2024, 2024
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Wet scavenging strongly influences aerosol lifetime and interactions but is a large uncertainty in global models. We present a method to identify meteorological variables relevant for estimating wet scavenging. During long-range transport over the tropical western Pacific, relative humidity and the frequency of humid conditions are better predictors of scavenging than precipitation. This method can be applied to other regions, and our findings can inform scavenging parameterizations in models.
Sarah Grawe, Conrad Jentzsch, Jonas Schaefer, Heike Wex, Stephan Mertes, and Frank Stratmann
Atmos. Meas. Tech., 16, 4551–4570, https://doi.org/10.5194/amt-16-4551-2023, https://doi.org/10.5194/amt-16-4551-2023, 2023
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Measurements of ice-nucleating particle (INP) concentrations are valuable for the simulation of cloud properties. In recent years, filter sampling in combination with offline INP measurements has become increasingly popular. However, most sampling is ground-based, and the vertical transport of INPs is not well quantified. The High-volume flow aERosol particle filter sAmpler (HERA) for applications on board aircraft was developed to expand the sparse dataset of INP concentrations at cloud level.
Claudio Crazzolara and Andreas Balthasar Held
Atmos. Meas. Tech. Discuss., https://doi.org/10.5194/amt-2023-182, https://doi.org/10.5194/amt-2023-182, 2023
Revised manuscript accepted for AMT
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Our manuscript describes the development of a collection device that can be used to collect airborne dust particles classified according to their size. This collection device is optimised for a special analysis method based on X-ray fluorescence, so that particles can be collected from the air and analysed with high sensitivity. This enables the determination of the content of heavy metals in the airborne particle fraction, which have a health-relevant significance.
Dimitri Castarède, Zoé Brasseur, Yusheng Wu, Zamin A. Kanji, Markus Hartmann, Lauri Ahonen, Merete Bilde, Markku Kulmala, Tuukka Petäjä, Jan B. C. Pettersson, Berko Sierau, Olaf Stetzer, Frank Stratmann, Birgitta Svenningsson, Erik Swietlicki, Quynh Thu Nguyen, Jonathan Duplissy, and Erik S. Thomson
Atmos. Meas. Tech., 16, 3881–3899, https://doi.org/10.5194/amt-16-3881-2023, https://doi.org/10.5194/amt-16-3881-2023, 2023
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Clouds play a key role in Earth’s climate by influencing the surface energy budget. Certain types of atmospheric aerosols, called ice-nucleating particles (INPs), induce the formation of ice in clouds and, thus, often initiate precipitation formation. The Portable Ice Nucleation Chamber 2 (PINCii) is a new instrument developed to study ice formation and to conduct ambient measurements of INPs, allowing us to investigate the sources and properties of the atmospheric aerosols that can act as INPs.
Markus Knoll, Martin Penz, Hannes Juchem, Christina Schmidt, Denis Pöhler, and Alexander Bergmann
EGUsphere, https://doi.org/10.5194/egusphere-2023-1279, https://doi.org/10.5194/egusphere-2023-1279, 2023
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Exhaust emissions from combustion-based vehicles are negatively affecting human health and our environment. In particular, a small share (< 20 %) of poorly maintained or tampered vehicles are responsible for the majority (60–90 %) of traffic-related emissions. The emissions from vehicles are currently not properly monitored during their lifetime. We present a roadside measurement technique, called point sampling, which can be used to monitor vehicle emissions throughout their life cycle.
Franz Martin Schnaiter, Claudia Linke, Eija Asmi, Henri Servomaa, Antti-Pekka Hyvärinen, Sho Ohata, Yutaka Kondo, and Emma Järvinen
Atmos. Meas. Tech., 16, 2753–2769, https://doi.org/10.5194/amt-16-2753-2023, https://doi.org/10.5194/amt-16-2753-2023, 2023
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Light-absorbing particles from combustion processes are important contributors to climate warming. Their highly variable spectral light absorption properties need to be monitored in the field. Commonly used methods show measurement artefacts that are difficult to correct. We introduce a new instrument that is based on the photoacoustic effect. Long-term operation in the Finnish Arctic demonstrates the applicability of the new instrument for unattended light absorption monitoring.
Dominik Stolzenburg, Tiia Laurila, Pasi Aalto, Joonas Vanhanen, Tuukka Petäjä, and Juha Kangasluoma
Atmos. Meas. Tech., 16, 2471–2483, https://doi.org/10.5194/amt-16-2471-2023, https://doi.org/10.5194/amt-16-2471-2023, 2023
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Size-distribution measurements of ultrafine particles are of special interest as they can be used to estimate the atmospheric significance of new particle formation, a process which is thought to influence the global climate. Here we show that improved counting statistics in size-distribution measurements through the usage of higher sampling flows can significantly reduce the uncertainties in such calculations.
Kamaljeet Kaur and Kerry E. Kelly
Atmos. Meas. Tech., 16, 2455–2470, https://doi.org/10.5194/amt-16-2455-2023, https://doi.org/10.5194/amt-16-2455-2023, 2023
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We evaluated the AlphaSense OPC-N3 and PMS5003 compared to federal equivalent method (FEM) PM10 measurements in the Salt Lake Valley during five dust events. Before correction, the OPC-N3 agreed well, but the PMS PM10 measurements correlated poorly with the FEM. After correcting the PMS with a PM2.5 / PM10 ratio-based factor, the PMS PM10 correlations improved significantly. This suggests the possibility of better resolved spatial estimates of PM10 using PMS measurements and PM2.5 / PM10 ratios.
Manuel Schöberl, Maximilian Dollner, Josef Gasteiger, Petra Seibert, Anne Tipka, and Bernadett Weinzierl
EGUsphere, https://doi.org/10.5194/egusphere-2023-439, https://doi.org/10.5194/egusphere-2023-439, 2023
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Transporting a representative aerosol sample to instrumentation inside a research aircraft remains a challenge due to losses or enhancements of particles in the aerosol sampling system. Here, we present sampling efficiencies and the cut-off diameter for the DLR Falcon aerosol sampling system as a function of true airspeed by comparing the in-cabin and the out-cabin particle number size distributions observed during the A-LIFE aircraft mission.
Balint Alfoldy, Asta Gregorič, Matic Ivančič, Irena Ježek, and Martin Rigler
Atmos. Meas. Tech., 16, 135–152, https://doi.org/10.5194/amt-16-135-2023, https://doi.org/10.5194/amt-16-135-2023, 2023
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Atmospheric concentrations and source apportionment (SA) of black carbon (BC) and CO2 were determined in an urban environment during a heating season. BC particles were attributed to two major sources: traffic and heating. The BC SA was implemented by an Aethalometer model used for the SA of CO2 supposing that the source-specific CO2 components are correlated with the corresponding BC. Source-specific emission factors were determined as a ratio of corresponding BC and CO2 components.
Christian Pilz, Sebastian Düsing, Birgit Wehner, Thomas Müller, Holger Siebert, Jens Voigtländer, and Michael Lonardi
Atmos. Meas. Tech., 15, 6889–6905, https://doi.org/10.5194/amt-15-6889-2022, https://doi.org/10.5194/amt-15-6889-2022, 2022
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Tethered balloon observations are highly valuable for aerosol studies in the lowest part of the atmosphere. This study presents a newly developed platform called CAMP with four aerosol instruments for balloon-borne measurements in the Arctic. Laboratory characterizations and evaluations of the instruments and results of a first field deployment are shown. A case study highlights CAMP's capabilities and the importance of airborne aerosol studies for interpretation of ground-based observations.
Weilun Zhao, Gang Zhao, Ying Li, Song Guo, Nan Ma, Lizi Tang, Zirui Zhang, and Chunsheng Zhao
Atmos. Meas. Tech., 15, 6807–6817, https://doi.org/10.5194/amt-15-6807-2022, https://doi.org/10.5194/amt-15-6807-2022, 2022
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A new method to determine black carbon mass size distribution (BCMSD) was proposed using the size-resolved absorption coefficient measured by an aerodynamic aerosol classifier in tandem with an aethalometer. This new method fills the gap in the high-time-resolution measurement of BCMSD ranging from upper submicron particle sizes to larger than 1 µm. This method can be applied to field measurement of BCMSD extensively for better understanding BC aging and better estimating the BC climate effect.
Antonis Dragoneas, Sergej Molleker, Oliver Appel, Andreas Hünig, Thomas Böttger, Markus Hermann, Frank Drewnick, Johannes Schneider, Ralf Weigel, and Stephan Borrmann
Atmos. Meas. Tech., 15, 5719–5742, https://doi.org/10.5194/amt-15-5719-2022, https://doi.org/10.5194/amt-15-5719-2022, 2022
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The ERICA is a specially designed aerosol particle mass spectrometer for in situ, real-time chemical composition analysis of aerosols. It can operate completely autonomously, in the absence of an instrument operator. Its design has enabled its operation under harsh conditions, like those experienced in the upper troposphere and lower stratosphere, aboard unpressurized high-altitude research aircraft. The instrument has successfully participated in several aircraft operations around the world.
Dimitrios Bousiotis, David C. S. Beddows, Ajit Singh, Molly Haugen, Sebastián Diez, Pete M. Edwards, Adam Boies, Roy M. Harrison, and Francis D. Pope
Atmos. Meas. Tech., 15, 4047–4061, https://doi.org/10.5194/amt-15-4047-2022, https://doi.org/10.5194/amt-15-4047-2022, 2022
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In the last decade, low-cost sensors have revolutionised the field of air quality monitoring. This paper extends the ability of low-cost sensors to not only measure air pollution, but also to understand where the pollution comes from. This "source apportionment" is a critical step in air quality management to allow for the mitigation of air pollution. The techniques developed in this paper have the potential for great impact in both research and industrial applications.
Luka Drinovec, Uroš Jagodič, Luka Pirker, Miha Škarabot, Mario Kurtjak, Kristijan Vidović, Luca Ferrero, Bradley Visser, Jannis Röhrbein, Ernest Weingartner, Daniel M. Kalbermatter, Konstantina Vasilatou, Tobias Bühlmann, Celine Pascale, Thomas Müller, Alfred Wiedensohler, and Griša Močnik
Atmos. Meas. Tech., 15, 3805–3825, https://doi.org/10.5194/amt-15-3805-2022, https://doi.org/10.5194/amt-15-3805-2022, 2022
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A new photothermal interferometer (PTAAM-2λ) for artefact-free determination of the aerosol absorption coefficient at two wavelengths is presented. The instrument is calibrated with NO2 and polydisperse nigrosin, resulting in very low uncertainties of the absorption coefficients: 4 % at 532 nm and 6 % at 1064 nm. The instrument’s performance makes the PTAAM-2λ a strong candidate for reference measurements of the aerosol absorption coefficient.
Markus Leiminger, Lukas Fischer, Sophia Brilke, Julian Resch, Paul Martin Winkler, Armin Hansel, and Gerhard Steiner
Atmos. Meas. Tech., 15, 3705–3720, https://doi.org/10.5194/amt-15-3705-2022, https://doi.org/10.5194/amt-15-3705-2022, 2022
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We developed an axial ion mobility classifier coupled to an atmospheric-pressure interface time-of-flight (APi-TOF) mass spectrometer to measure size-segregated atmospheric ions. We characterize the performance of the novel instrument with bipolar-electrospray-generated ion mobility standards and compare the results with CFD simulations and a simplified numerical particle-tracking model. Ultimately, we report first mass–mobility measurements of atmospheric ions in Innsbruck, Austria.
Andreas Hünig, Oliver Appel, Antonis Dragoneas, Sergej Molleker, Hans-Christian Clemen, Frank Helleis, Thomas Klimach, Franziska Köllner, Thomas Böttger, Frank Drewnick, Johannes Schneider, and Stephan Borrmann
Atmos. Meas. Tech., 15, 2889–2921, https://doi.org/10.5194/amt-15-2889-2022, https://doi.org/10.5194/amt-15-2889-2022, 2022
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We have serially combined the two well-established methods for in situ real-time measurement of fine particle chemical composition, the single-particle laser ablation method and the flash evaporation with electron impact ionization method, into a novel instrument. Here we present the design; instrument characteristics, as derived from laboratory and field measurements; and results from the first field deployment during the 2017 StratoClim aircraft campaign.
Christopher D. Wallis, Mason D. Leandro, Patrick Y. Chuang, and Anthony S. Wexler
Atmos. Meas. Tech., 15, 2547–2556, https://doi.org/10.5194/amt-15-2547-2022, https://doi.org/10.5194/amt-15-2547-2022, 2022
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Measuring emissions from stacks requires techniques to address a broad range of conditions and measurement challenges. Here we describe an instrument package held by a crane above a stack to characterize both wet droplet and dried aerosol emissions from cooling tower spray drift in situ. The instrument package characterizes the velocity, size distribution, and concentration of the wet droplet emissions and the mass concentration and elemental composition of the dried PM2.5 and PM10 emissions.
Karin Ardon-Dryer, Mary C. Kelley, Xia Xueting, and Yuval Dryer
Atmos. Meas. Tech., 15, 2345–2360, https://doi.org/10.5194/amt-15-2345-2022, https://doi.org/10.5194/amt-15-2345-2022, 2022
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The Aerosol Research Observation Station (AEROS) located in West Texas was designed to continuously measure atmospheric particles, including different particulate matter sizes, total particle number concentration, and size distribution. This article provides a description of AEROS as well as an intercomparison of the different instruments using laboratory and atmospheric particles, showing similar concentration as well to distinguish between various pollution events (natural vs. anthropogenic).
Adam T. Ahern, Frank Erdesz, Nicholas L. Wagner, Charles A. Brock, Ming Lyu, Kyra Slovacek, Richard H. Moore, Elizabeth B. Wiggins, and Daniel M. Murphy
Atmos. Meas. Tech., 15, 1093–1105, https://doi.org/10.5194/amt-15-1093-2022, https://doi.org/10.5194/amt-15-1093-2022, 2022
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Particles in the atmosphere play a significant role in climate change by scattering light back into space, reducing the amount of energy available to be absorbed by greenhouse gases. We built a new instrument to measure what direction light is scattered by particles, e.g., wildfire smoke. This is important because, depending on the angle of the sun, some particles scatter light into space (cooling the planet), but some light is also scattered towards the Earth (not cooling the planet).
Yuya Kobayashi and Nobuyuki Takegawa
Atmos. Meas. Tech., 15, 833–844, https://doi.org/10.5194/amt-15-833-2022, https://doi.org/10.5194/amt-15-833-2022, 2022
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We propose a new method to quantify particulate sodium and potassium salts (nitrate, chloride, and sulfate) by using a refractory aerosol thermal desorption mass spectrometer (rTDMS). The combination of a graphite particle collector and a carbon dioxide laser enables high desorption temperature. Laboratory experiments showed that major ion signals originating from sodium or potassium salts were clearly detected, associated with the increase in the desorption temperature by laser heating.
James R. Ouimette, William C. Malm, Bret A. Schichtel, Patrick J. Sheridan, Elisabeth Andrews, John A. Ogren, and W. Patrick Arnott
Atmos. Meas. Tech., 15, 655–676, https://doi.org/10.5194/amt-15-655-2022, https://doi.org/10.5194/amt-15-655-2022, 2022
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We show that the low-cost PurpleAir sensor can be characterized as a cell-reciprocal nephelometer. At two very different locations (Mauna Loa Observatory in Hawaii and the Table Mountain rural site in Colorado), the PurpleAir measurements are highly correlated with the submicrometer aerosol scattering coefficient measured by a research-grade integrating nephelometer. These results imply that, with care, PurpleAir data may be used to evaluate climate and air quality models.
Steven G. Howell, Steffen Freitag, Amie Dobracki, Nikolai Smirnow, and Arthur J. Sedlacek III
Atmos. Meas. Tech., 14, 7381–7404, https://doi.org/10.5194/amt-14-7381-2021, https://doi.org/10.5194/amt-14-7381-2021, 2021
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Small particles in the air have important effects on visibility, clouds, and human health. For the ORACLES project we got a new particle sizing instrument that is fast, works over the most important particle sizes, and avoids some of the issues that plague other optical particle sizers. Unfortunately it sees some particles much smaller than they really are, likely because they heat up and evaporate. We show a crude correction and speculate why these particles heat up much more than expected.
Jeffrey K. Bean
Atmos. Meas. Tech., 14, 7369–7379, https://doi.org/10.5194/amt-14-7369-2021, https://doi.org/10.5194/amt-14-7369-2021, 2021
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Understanding and improving the quality of data generated from low-cost air quality sensors are crucial steps in using these sensors. This work investigates how averaging time, choice of reference instrument, and the observation of higher pollutant concentrations can impact the perceived performance of low-cost sensors in an evaluation. The influence of these factors should be considered when comparing one sensor to another or determining if a sensor can produce data that fit a specific need.
Fan Mei, Steven Spielman, Susanne Hering, Jian Wang, Mikhail S. Pekour, Gregory Lewis, Beat Schmid, Jason Tomlinson, and Maynard Havlicek
Atmos. Meas. Tech., 14, 7329–7340, https://doi.org/10.5194/amt-14-7329-2021, https://doi.org/10.5194/amt-14-7329-2021, 2021
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This study focuses on understanding a versatile water-based condensation particle counter (vWCPC 3789) performance under various ambient pressure conditions (500–1000 hPa). A vWCPC has the advantage of avoiding health and safety concerns. However, its performance characterization under low pressure is rare but crucial for ensuring successful airborne deployment. This paper provides advanced knowledge of operating a vWCPC 3789 to capture the spatial variations of atmospheric aerosols.
Rebecca A. Wernis, Nathan M. Kreisberg, Robert J. Weber, Yutong Liang, John Jayne, Susanne Hering, and Allen H. Goldstein
Atmos. Meas. Tech., 14, 6533–6550, https://doi.org/10.5194/amt-14-6533-2021, https://doi.org/10.5194/amt-14-6533-2021, 2021
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cTAG is a new scientific instrument that measures concentrations of organic chemicals in the atmosphere. cTAG is the first instrument capable of measuring small, light chemicals as well as heavier chemicals and everything in between on a single detector, every hour. In this work we explain how cTAG works and some of the tests we performed to verify that it works properly and reliably. We also present measurements of alkanes that suggest they have three dominant sources in a Bay Area suburb.
Linghan Zeng, Amy P. Sullivan, Rebecca A. Washenfelder, Jack Dibb, Eric Scheuer, Teresa L. Campos, Joseph M. Katich, Ezra Levin, Michael A. Robinson, and Rodney J. Weber
Atmos. Meas. Tech., 14, 6357–6378, https://doi.org/10.5194/amt-14-6357-2021, https://doi.org/10.5194/amt-14-6357-2021, 2021
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Three online systems for measuring water-soluble brown carbon are compared. A mist chamber and two different particle-into-liquid samplers were deployed on separate research aircraft targeting wildfires and followed a similar detection method using a long-path liquid waveguide with a spectrometer to measure the light absorption from 300 to 700 nm. Detection limits, signal hysteresis and other sampling issues are compared, and further improvements of these liquid-based systems are provided.
Zixia Liu, Martin Osborne, Karen Anderson, Jamie D. Shutler, Andy Wilson, Justin Langridge, Steve H. L. Yim, Hugh Coe, Suresh Babu, Sreedharan K. Satheesh, Paquita Zuidema, Tao Huang, Jack C. H. Cheng, and James Haywood
Atmos. Meas. Tech., 14, 6101–6118, https://doi.org/10.5194/amt-14-6101-2021, https://doi.org/10.5194/amt-14-6101-2021, 2021
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This paper first validates the performance of an advanced aerosol observation instrument POPS against a reference instrument and examines any biases introduced by operating it on a quadcopter drone. The results show the POPS performs relatively well on the ground. The impact of the UAV rotors on the POPS is small at low wind speeds, but when operating under higher wind speeds, larger discrepancies occur. It appears that the POPS measures sub-micron aerosol particles more accurately on the UAV.
Eric A. Wendt, Casey Quinn, Christian L'Orange, Daniel D. Miller-Lionberg, Bonne Ford, Jeffrey R. Pierce, John Mehaffy, Michael Cheeseman, Shantanu H. Jathar, David H. Hagan, Zoey Rosen, Marilee Long, and John Volckens
Atmos. Meas. Tech., 14, 6023–6038, https://doi.org/10.5194/amt-14-6023-2021, https://doi.org/10.5194/amt-14-6023-2021, 2021
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Fine particulate matter air pollution is one of the leading contributors to adverse health outcomes on the planet. Here, we describe the design and validation of a low-cost, compact, and autonomous instrument capable of measuring particulate matter levels directly, via mass sampling, and optically, via mass and sunlight extinction measurements. We demonstrate the instrument's accuracy relative to reference measurements and its potential for community-level sampling.
Jiaoshi Zhang, Steven Spielman, Yang Wang, Guangjie Zheng, Xianda Gong, Susanne Hering, and Jian Wang
Atmos. Meas. Tech., 14, 5625–5635, https://doi.org/10.5194/amt-14-5625-2021, https://doi.org/10.5194/amt-14-5625-2021, 2021
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In this study, we present a newly developed instrument, the humidity-controlled fast integrated mobility spectrometer (HFIMS), for fast measurements of aerosol hygroscopic growth. The HFIMS can measure the distributions of particle hygroscopic growth factors at six diameters from 35 to 265 nm under five RH levels from 20 to 85 % within 25 min. The HFIMS significantly advances our capability of characterizing the hygroscopic growth of atmospheric aerosols over a wide range of relative humidities.
Johannes Passig, Julian Schade, Robert Irsig, Lei Li, Xue Li, Zhen Zhou, Thomas Adam, and Ralf Zimmermann
Atmos. Meas. Tech., 14, 4171–4185, https://doi.org/10.5194/amt-14-4171-2021, https://doi.org/10.5194/amt-14-4171-2021, 2021
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Ships are major sources of air pollution; however, monitoring of ship emissions outside harbours is a challenging task. We optimized single-particle mass spectrometry (SPMS) for the detection of bunker fuel emissions and demonstrate the detection of individual ship plumes from more than 10 km in distance. The approach works independently of background air pollution and also when ships use exhaust-cleaning scrubbers. We discuss the potential and limits of SPMS-based monitoring of ship plumes.
Mengying Bao, Yan-Lin Zhang, Fang Cao, Yu-Chi Lin, Yuhang Wang, Xiaoyan Liu, Wenqi Zhang, Meiyi Fan, Feng Xie, Robert Cary, Joshua Dixon, and Lihua Zhou
Atmos. Meas. Tech., 14, 4053–4068, https://doi.org/10.5194/amt-14-4053-2021, https://doi.org/10.5194/amt-14-4053-2021, 2021
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We introduce a two-wavelength method for brown C measurements with a modified Sunset carbon analyzer. We defined the enhanced concentrations and gave the possibility of providing an indicator of brown C. Compared with the strong local sources of organic and elemental C, we found that differences in EC mainly originated from regional transport. Biomass burning emissions significantly contributed to high differences in EC concentrations during the heavy biomass burning periods.
Candice L. Sirmollo, Don R. Collins, Jordan M. McCormick, Cassandra F. Milan, Matthew H. Erickson, James H. Flynn, Rebecca J. Sheesley, Sascha Usenko, Henry W. Wallace, Alexander A. T. Bui, Robert J. Griffin, Matthew Tezak, Sean M. Kinahan, and Joshua L. Santarpia
Atmos. Meas. Tech., 14, 3351–3370, https://doi.org/10.5194/amt-14-3351-2021, https://doi.org/10.5194/amt-14-3351-2021, 2021
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The newly developed portable 1 m3 CAGE chamber systems were characterized using data acquired during a 2-month field study in 2016 in a forested area north of Houston, TX, USA. Concentrations of several oxidant and organic compounds measured in the chamber were found to closely agree with those calculated with a zero-dimensional model. By tracking the modes of injected monodisperse particles, a pattern change was observed for hourly averaged growth rates between late summer and early fall.
Ningjin Xu and Don R. Collins
Atmos. Meas. Tech., 14, 2891–2906, https://doi.org/10.5194/amt-14-2891-2021, https://doi.org/10.5194/amt-14-2891-2021, 2021
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Oxidation flow reactors (OFRs) are frequently used to study atmospheric chemistry and aerosol formation by accelerating by up to 10 000 times the reactions that can take hours, days, or even weeks in the atmosphere. Here we present the design and evaluation of a new all-Teflon OFR. The computational, laboratory, and field use data we present demonstrate that the PFA OFR is suitable for a range of applications, including the study of rapidly changing ambient concentrations.
Lars E. Kalnajs, Sean M. Davis, J. Douglas Goetz, Terry Deshler, Sergey Khaykin, Alex St. Clair, Albert Hertzog, Jerome Bordereau, and Alexey Lykov
Atmos. Meas. Tech., 14, 2635–2648, https://doi.org/10.5194/amt-14-2635-2021, https://doi.org/10.5194/amt-14-2635-2021, 2021
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This work introduces a novel instrument system for high-resolution atmospheric profiling, which lowers and retracts a suspended instrument package beneath drifting long-duration balloons. During a 100 d circumtropical flight, the instrument collected over a hundred 2 km profiles of temperature, water vapor, clouds, and aerosol at 1 m resolution, yielding unprecedented geographic sampling and vertical resolution measurements of the tropical tropopause layer.
Demetrios Pagonis, Pedro Campuzano-Jost, Hongyu Guo, Douglas A. Day, Melinda K. Schueneman, Wyatt L. Brown, Benjamin A. Nault, Harald Stark, Kyla Siemens, Alex Laskin, Felix Piel, Laura Tomsche, Armin Wisthaler, Matthew M. Coggon, Georgios I. Gkatzelis, Hannah S. Halliday, Jordan E. Krechmer, Richard H. Moore, David S. Thomson, Carsten Warneke, Elizabeth B. Wiggins, and Jose L. Jimenez
Atmos. Meas. Tech., 14, 1545–1559, https://doi.org/10.5194/amt-14-1545-2021, https://doi.org/10.5194/amt-14-1545-2021, 2021
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We describe the airborne deployment of an extractive electrospray time-of-flight mass spectrometer (EESI-MS). The instrument provides a quantitative 1 Hz measurement of the chemical composition of organic aerosol up to altitudes of
7 km, with single-compound detection limits as low as 50 ng per standard cubic meter.
Xiaona Shang, Ling Li, Xinlian Zhang, Huihui Kang, Guodong Sui, Gehui Wang, Xingnan Ye, Hang Xiao, and Jianmin Chen
Atmos. Meas. Tech., 14, 1037–1045, https://doi.org/10.5194/amt-14-1037-2021, https://doi.org/10.5194/amt-14-1037-2021, 2021
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Oxidative stress can be used to evaluate not only adverse health effects but also adverse ecological effects. However, little research uses eco-toxicological assay to assess the risks posed by particle matter to non-human biomes. One important reason might be that the concentration of toxic components of atmospheric particles is far below the high detection limit of eco-toxic measurement. To solve the rapid detection problem, we extended a VACES for ecotoxicity aerosol measurement.
Joan Stude, Heinfried Aufmhoff, Hans Schlager, Markus Rapp, Frank Arnold, and Boris Strelnikov
Atmos. Meas. Tech., 14, 983–993, https://doi.org/10.5194/amt-14-983-2021, https://doi.org/10.5194/amt-14-983-2021, 2021
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In this paper we describe the instrument ROMARA and show data from the first flight on a research rocket.
On the way through the atmosphere, the instrument detects positive and negative, natural occurring ions before returning back to ground.
ROMARA was successfully launched together with other instruments into a special radar echo.
We detected typical, light ions of positive and negative charge and heavy negative ions, but no heavy positive ions.
Rob L. Modini, Joel C. Corbin, Benjamin T. Brem, Martin Irwin, Michele Bertò, Rosaria E. Pileci, Prodromos Fetfatzis, Kostas Eleftheriadis, Bas Henzing, Marcel M. Moerman, Fengshan Liu, Thomas Müller, and Martin Gysel-Beer
Atmos. Meas. Tech., 14, 819–851, https://doi.org/10.5194/amt-14-819-2021, https://doi.org/10.5194/amt-14-819-2021, 2021
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Extinction-minus-scattering is an important method for measuring aerosol light absorption, but its application in the field presents a number of challenges. A recently developed instrument based on this method – the CAPS PMssa – has the potential to overcome some of these challenges. We present a compilation of theory, lab measurements, and field examples to characterize this instrument and show the conditions under which it can deliver reliable absorption measurements for atmospheric aerosols.
Carolyn E. Jordan, Ryan M. Stauffer, Brian T. Lamb, Charles H. Hudgins, Kenneth L. Thornhill, Gregory L. Schuster, Richard H. Moore, Ewan C. Crosbie, Edward L. Winstead, Bruce E. Anderson, Robert F. Martin, Michael A. Shook, Luke D. Ziemba, Andreas J. Beyersdorf, Claire E. Robinson, Chelsea A. Corr, and Maria A. Tzortziou
Atmos. Meas. Tech., 14, 695–713, https://doi.org/10.5194/amt-14-695-2021, https://doi.org/10.5194/amt-14-695-2021, 2021
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First field data from a custom-built in situ instrument measuring hyperspectral (300–700 nm, 0.8 nm resolution) ambient atmospheric aerosol extinction are presented. The advantage of this capability is that it can be directly linked to other in situ techniques that measure physical and chemical properties of atmospheric aerosols. Second-order polynomials provided a better fit to the data than traditional power law fits, yielding greater discrimination among distinct ambient aerosol populations.
Carolyn E. Jordan, Ryan M. Stauffer, Brian T. Lamb, Michael Novak, Antonio Mannino, Ewan C. Crosbie, Gregory L. Schuster, Richard H. Moore, Charles H. Hudgins, Kenneth L. Thornhill, Edward L. Winstead, Bruce E. Anderson, Robert F. Martin, Michael A. Shook, Luke D. Ziemba, Andreas J. Beyersdorf, Claire E. Robinson, Chelsea A. Corr, and Maria A. Tzortziou
Atmos. Meas. Tech., 14, 715–736, https://doi.org/10.5194/amt-14-715-2021, https://doi.org/10.5194/amt-14-715-2021, 2021
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In situ measurements of ambient atmospheric aerosol hyperspectral (300–700 nm) optical properties (extinction, total absorption, water- and methanol-soluble absorption) were observed around the Korean peninsula. Such in situ observations provide a direct link between ambient aerosol optical properties and their physicochemical properties. The benefit of hyperspectral measurements is evident as simple mathematical functions could not fully capture the observed spectral detail of ambient aerosols.
Cyril Brunner and Zamin A. Kanji
Atmos. Meas. Tech., 14, 269–293, https://doi.org/10.5194/amt-14-269-2021, https://doi.org/10.5194/amt-14-269-2021, 2021
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Subvisual microscopic particles in the atmosphere are needed to act as seeds for cloud droplets or ice crystals to form. The microscopic particles, called ice-nucleating particles (INPs), form ice crystals and are rare, and their properties are not well understood, in part because measuring them is challenging and time consuming, and to date has not been automated. Here, we present the first online instrument that can continuously and autonomously measure INP concentration at 243 K.
Adnan Masic, Dzevad Bibic, Boran Pikula, Almir Blazevic, Jasna Huremovic, and Sabina Zero
Atmos. Meas. Tech., 13, 6427–6443, https://doi.org/10.5194/amt-13-6427-2020, https://doi.org/10.5194/amt-13-6427-2020, 2020
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Optical-based particulate matter sensors offer some advantages: price (especially low-cost sensors), time and space resolution, but they are less accurate than reference instruments. Understanding their performance and limitations is crucial for wider adoption. This is a case study for strong and mild air pollution done in Sarajevo, Bosnia-Herzegovina. Tested optical sensors were found to be generally acceptable in this study, but proper calibration is required for getting reliable data.
Hans-Christian Clemen, Johannes Schneider, Thomas Klimach, Frank Helleis, Franziska Köllner, Andreas Hünig, Florian Rubach, Stephan Mertes, Heike Wex, Frank Stratmann, André Welti, Rebecca Kohl, Fabian Frank, and Stephan Borrmann
Atmos. Meas. Tech., 13, 5923–5953, https://doi.org/10.5194/amt-13-5923-2020, https://doi.org/10.5194/amt-13-5923-2020, 2020
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We improved the efficiency of a single-particle mass spectrometer with a newly developed aerodynamic lens system, delayed ion extraction, and better electric shielding. The new components result in significantly improved particle analysis and sample statistics. This is particularly important for measurements of low-number-density particles, such as ice-nucleating particles, and for aircraft-based measurements at high altitudes or where high temporal and spatial resolution is required.
Karin Ardon-Dryer, Yuval Dryer, Jake N. Williams, and Nastaran Moghimi
Atmos. Meas. Tech., 13, 5441–5458, https://doi.org/10.5194/amt-13-5441-2020, https://doi.org/10.5194/amt-13-5441-2020, 2020
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The PurpleAir PA-II is a low-cost sensor for monitoring changes in the concentrations of particulate matter of various sizes. This study examined the behaviour of multiple PA-II units in four locations in the USA under atmospheric conditions when exposed to a variety of pollutants and different PM2.5 concentrations. The PA-II unit is a promising tool for measuring PM2.5 concentrations and identifying relative concentration changes, as long as the
PA-II PM2.5 values can be corrected.
Cui-Ping Su, Xing Peng, Xiao-Feng Huang, Li-Wu Zeng, Li-Ming Cao, Meng-Xue Tang, Yao Chen, Bo Zhu, Yishi Wang, and Ling-Yan He
Atmos. Meas. Tech., 13, 5407–5422, https://doi.org/10.5194/amt-13-5407-2020, https://doi.org/10.5194/amt-13-5407-2020, 2020
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Online instruments have been widely applied for the measurement of PM2.5 and its chemical components; however, these instruments have a major shortcoming in terms of the limited number (or lack) of species in field measurements. To this end, a new mass closure PM2.5 online-integrated system was developed and applied in this work to achieve more comprehensive information on chemical species in PM2.5, thus providing a powerful tool for PM2.5 long-term daily measurement and source apportionment.
Anna K. Tobler, Alicja Skiba, Dongyu S. Wang, Philip Croteau, Katarzyna Styszko, Jarosław Nęcki, Urs Baltensperger, Jay G. Slowik, and André S. H. Prévôt
Atmos. Meas. Tech., 13, 5293–5301, https://doi.org/10.5194/amt-13-5293-2020, https://doi.org/10.5194/amt-13-5293-2020, 2020
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Some quadrupole aerosol chemical speciation monitors (Q-ACSMs) have had issues with the quantification of particulate chloride, resulting in apparent negative chloride concentrations. We can show that this is due to the different behavior of Cl+ and HCl+, and we present a correction for the more accurate quantification of chloride. The correction can be applied to measurements in environments where the particulate chloride is dominated by NH4Cl.
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Short summary
Energetic photons, such as ultraviolet light, are able to eject electrons from a material surface, thus creating an electrical current, also called a photocurrent. A proper estimation of this photocurrent can be crucial for space- or rocket-borne particle detectors, as it can dominate over the currents that are of scientific interest (induced by charged particles, for example). This article outlines the design for photocurrent modelling and for experimental confirmation in a laboratory.
Energetic photons, such as ultraviolet light, are able to eject electrons from a material...
