Articles | Volume 12, issue 4
https://doi.org/10.5194/amt-12-2445-2019
© Author(s) 2019. This work is distributed under
the Creative Commons Attribution 4.0 License.
the Creative Commons Attribution 4.0 License.
https://doi.org/10.5194/amt-12-2445-2019
© Author(s) 2019. This work is distributed under
the Creative Commons Attribution 4.0 License.
the Creative Commons Attribution 4.0 License.
Research article
| 
17 Apr 2019
Research article |
| 17 Apr 2019
| 17 Apr 2019
Atomic oxygen number densities in the mesosphere–lower thermosphere region measured by solid electrolyte sensors on WADIS-2
Martin Eberhart
CORRESPONDING AUTHOR
Institute of Space Systems, University of Stuttgart, Stuttgart, Germany
Stefan Löhle
Institute of Space Systems, University of Stuttgart, Stuttgart, Germany
Boris Strelnikov
Leibniz-Institute of Atmospheric Physics, University of Rostock, Kühlungsborn, Germany
Jonas Hedin
Department of Meteorology (MISU), Stockholm University, Stockholm, Sweden
Mikhail Khaplanov
Department of Meteorology (MISU), Stockholm University, Stockholm, Sweden
deceased
Stefanos Fasoulas
Institute of Space Systems, University of Stuttgart, Stuttgart, Germany
Jörg Gumbel
Department of Meteorology (MISU), Stockholm University, Stockholm, Sweden
Franz-Josef Lübken
Leibniz-Institute of Atmospheric Physics, University of Rostock, Kühlungsborn, Germany
Markus Rapp
Institute of Atmospheric Physics, German Aerospace Center, Oberpfaffenhofen, Germany
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Robert Reichert, Bernd Kaifler, Natalie Kaifler, Markus Rapp, Pierre-Dominique Pautet, Michael J. Taylor, Alexander Kozlovsky, Mark Lester, and Rigel Kivi
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Ralph Latteck, Toralf Renkwitz, and Boris Strelnikov
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Boris Strelnikov, Martin Eberhart, Martin Friedrich, Jonas Hedin, Mikhail Khaplanov, Gerd Baumgarten, Bifford P. Williams, Tristan Staszak, Heiner Asmus, Irina Strelnikova, Ralph Latteck, Mykhaylo Grygalashvyly, Franz-Josef Lübken, Josef Höffner, Raimund Wörl, Jörg Gumbel, Stefan Löhle, Stefanos Fasoulas, Markus Rapp, Aroh Barjatya, Michael J. Taylor, and Pierre-Dominique Pautet
Atmos. Chem. Phys., 19, 11443–11460, https://doi.org/10.5194/acp-19-11443-2019, https://doi.org/10.5194/acp-19-11443-2019, 2019
Short summary
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Jens Faber, Michael Gerding, Andreas Schneider, Andreas Dörnbrack, Henrike Wilms, Johannes Wagner, and Franz-Josef Lübken
Atmos. Meas. Tech., 12, 4191–4210, https://doi.org/10.5194/amt-12-4191-2019, https://doi.org/10.5194/amt-12-4191-2019, 2019
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Atmospheric measurements on rising balloons can be compromised by the balloon's wake. The aim of this study is to provide a tool for assessing the likelihood of encountering the balloon's wake at the position of the gondola. This includes an uncertainty analysis of the calculation and a retrieval of vertical winds. We find an average wake encounter probability of 28 % for a standard radiosonde. Additionally, we evaluate the influence of wake from smaller objects on turbulence measurements.
Jacob Zalach, Christian von Savigny, Arvid Langenbach, Gerd Baumgarten, Franz-Josef Lübken, and Adam Bourassa
Atmos. Meas. Tech. Discuss., https://doi.org/10.5194/amt-2019-267, https://doi.org/10.5194/amt-2019-267, 2019
Revised manuscript not accepted
Arvid Langenbach, Gerd Baumgarten, Jens Fiedler, Franz-Josef Lübken, Christian von Savigny, and Jacob Zalach
Atmos. Meas. Tech., 12, 4065–4076, https://doi.org/10.5194/amt-12-4065-2019, https://doi.org/10.5194/amt-12-4065-2019, 2019
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Stratospheric aerosol backscatter ratios in the Arctic using Rayleigh, Mie and Raman backscattered signals were calculated. A backscatter ratio calculation during daytime was performed for the first time. Sharp aerosol layers thinner than 1 km over several days were observed. The seasonal cycle of stratospheric background aerosol in high latitudes including the summer months was calculated for the first time. Top altitude of the aerosol layer was found to reach up to 34 km, especially in summer.
Uwe Berger, Gerd Baumgarten, Jens Fiedler, and Franz-Josef Lübken
Atmos. Chem. Phys., 19, 4685–4702, https://doi.org/10.5194/acp-19-4685-2019, https://doi.org/10.5194/acp-19-4685-2019, 2019
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In this paper we present a new description of statistical probability density functions (pdfs) of polar mesospheric clouds (PMC). We derive a new class of pdfs that describes successfully the probability statistic of ALOMAR lidar observations of different ice parameters. As a main advantage the new method allows us to connect different observational PMC distributions of lidar and satellite data, and also to compare with distributions from ice model studies.
Mario Nachbar, Henrike Wilms, Denis Duft, Tasha Aylett, Kensei Kitajima, Takuya Majima, John M. C. Plane, Markus Rapp, and Thomas Leisner
Atmos. Chem. Phys., 19, 4311–4322, https://doi.org/10.5194/acp-19-4311-2019, https://doi.org/10.5194/acp-19-4311-2019, 2019
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Polar mesospheric clouds (PMC) are water ice clouds forming on nanoparticles in the polar summer mesopause. We investigate the impact of solar radiation on PMC formation in the laboratory. We show that Mie theory calculations combined with an equilibrium temperature model presented in this work predict the warming of the particles very well. Using this model we demonstrate that the impact of solar radiation on ice particle formation is significantly lower than previously assumed.
Mykhaylo Grygalashvyly, Martin Eberhart, Jonas Hedin, Boris Strelnikov, Franz-Josef Lübken, Markus Rapp, Stefan Löhle, Stefanos Fasoulas, Mikhail Khaplanov, Jörg Gumbel, and Ekaterina Vorobeva
Atmos. Chem. Phys., 19, 1207–1220, https://doi.org/10.5194/acp-19-1207-2019, https://doi.org/10.5194/acp-19-1207-2019, 2019
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Based on rocket-borne true common volume observations of atomic oxygen, atmospheric band emission (762 nm), and background atmosphere density and temperature, one-step, two-step, and combined mechanisms of
O2(b1Σg+) formation were analyzed. We found new coefficients for the fit function based on self-consistent temperature, atomic oxygen, and volume emission observations. This can be used for atmospheric band volume emission modeling or the estimation of atomic oxygen by known volume emission.
Raimund Wörl, Boris Strelnikov, Timo P. Viehl, Josef Höffner, Pierre-Dominique Pautet, Michael J. Taylor, Yucheng Zhao, and Franz-Josef Lübken
Atmos. Chem. Phys., 19, 77–88, https://doi.org/10.5194/acp-19-77-2019, https://doi.org/10.5194/acp-19-77-2019, 2019
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Simultaneous temperature measurements during the WADIS-2 rocket campaign are used to investigate the thermal structure of the mesopause region. Vertically and horizontally resolved in situ and remote measurements are in good agreement and show dominating long-term and large-scale waves with periods of 24 h and higher tidal harmonics. Only a few gravity waves with periods shorter than 6 h and small amplitudes are there.
Michael Gerding, Jochen Zöllner, Marius Zecha, Kathrin Baumgarten, Josef Höffner, Gunter Stober, and Franz-Josef Lübken
Atmos. Chem. Phys., 18, 15569–15580, https://doi.org/10.5194/acp-18-15569-2018, https://doi.org/10.5194/acp-18-15569-2018, 2018
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We describe the first comparative study of noctilucent clouds (NLCs) and mesospheric summer echoes at midlatitudes. Therefore, this study compares fresh clouds (small particles) with fully evolved clouds in the mesosphere, hinting at their evolution. It is shown that, in contrast to higher latitudes, here only a thin layer of fresh particles exist above the NLCs. This gives evidence that NLCs are not formed locally but are typically advected. This needs to be acknowledged in trend studies.
Gabriel Giono, Boris Strelnikov, Heiner Asmus, Tristan Staszak, Nickolay Ivchenko, and Franz-Josef Lübken
Atmos. Meas. Tech., 11, 5299–5314, https://doi.org/10.5194/amt-11-5299-2018, https://doi.org/10.5194/amt-11-5299-2018, 2018
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Energetic photons, such as ultraviolet light, are able to eject electrons from a material surface, thus creating an electrical current, also called a photocurrent. A proper estimation of this photocurrent can be crucial for space- or rocket-borne particle detectors, as it can dominate over the currents that are of scientific interest (induced by charged particles, for example). This article outlines the design for photocurrent modelling and for experimental confirmation in a laboratory.
Andreas Dörnbrack, Sonja Gisinger, Natalie Kaifler, Tanja Christina Portele, Martina Bramberger, Markus Rapp, Michael Gerding, Jens Faber, Nedjeljka Žagar, and Damjan Jelić
Atmos. Chem. Phys., 18, 12915–12931, https://doi.org/10.5194/acp-18-12915-2018, https://doi.org/10.5194/acp-18-12915-2018, 2018
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A deep upper-air sounding stimulated the current investigation of internal gravity waves excited during a minor sudden stratospheric warming (SSW) in the Arctic winter 2015/16. The analysis of the radiosonde profile revealed large kinetic and potential energies in the upper stratosphere without any simultaneous enhancement of upper tropospheric and lower stratospheric values. In combination with high-resolution meteorological analyses we identified an elevated source of gravity wave excitation.
Gerald A. Lehmacher, Miguel F. Larsen, Richard L. Collins, Aroh Barjatya, and Boris Strelnikov
Ann. Geophys., 36, 1099–1116, https://doi.org/10.5194/angeo-36-1099-2018, https://doi.org/10.5194/angeo-36-1099-2018, 2018
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We used sounding rockets to obtain four high-resolution temperature profiles in the mesosphere over a limited area. We found consistent deep isothermal and adiabatic layers, but variable and finely structured turbulence preferentially in the lower stable mesosphere. Accompanying tracer releases showed horizontal winds in the lower thermosphere with extreme shears and 200 m s−1 winds under moderately disturbed geomagnetic conditions, and convection-like structures just below the mesopause.
Francie Schmidt, Gerd Baumgarten, Uwe Berger, Jens Fiedler, and Franz-Josef Lübken
Atmos. Chem. Phys., 18, 8893–8908, https://doi.org/10.5194/acp-18-8893-2018, https://doi.org/10.5194/acp-18-8893-2018, 2018
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Local time variations of polar mesospheric clouds (PMCs) in the Northern Hemisphere are studied using a combination of a global circulation model and a microphysical model. We investigate the brightness, altitude, and occurrence of the clouds and find a good agreement between model and observations. The variations are caused by tidal structures in background parameters. The temperature varies by about 2 K and water vapor by about 3 ppmv at the altitude of ice particle sublimation near 81.5 km.
Rolf Rüfenacht, Gerd Baumgarten, Jens Hildebrand, Franziska Schranz, Vivien Matthias, Gunter Stober, Franz-Josef Lübken, and Niklaus Kämpfer
Atmos. Meas. Tech., 11, 1971–1987, https://doi.org/10.5194/amt-11-1971-2018, https://doi.org/10.5194/amt-11-1971-2018, 2018
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Wind information throughout the middle-atmosphere is crucial for the understanding of atmospheric dynamics but became available only recently, thanks to developments in remote sensing and modelling approaches. We present the first thorough assessment of the quality of the wind estimates by comparing co-located observations from lidar and microwave radiometry and opposing them to the major atmospheric models. Moreover we evaluated a new approach for measuring mesopause region wind by radiometry.
Qiang Li, Markus Rapp, Gunter Stober, and Ralph Latteck
Ann. Geophys., 36, 577–586, https://doi.org/10.5194/angeo-36-577-2018, https://doi.org/10.5194/angeo-36-577-2018, 2018
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With the powerful MAARSY radar, we detected 3D wind fields and the vertical winds show a non-Gaussian distribution. We further obtained the frequency spectrum of vertical wind. The distribution of the spectral slopes under different wind conditions is derived and their comparisons with the background horizontal winds show that the spectra become steeper with increasing wind velocities under quiet conditions, approach a slope of −5/3 at 10 m/s and then maintain this slope for even stronger winds.
Markus Rapp, Andreas Dörnbrack, and Bernd Kaifler
Atmos. Meas. Tech., 11, 1031–1048, https://doi.org/10.5194/amt-11-1031-2018, https://doi.org/10.5194/amt-11-1031-2018, 2018
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Temperature profiles from operational weather satellites are used to determine the global distribution of gravity wave activity. This is an important information to constrain global climate models. The quality of this data set is assessed by
systematic comparison to model fields from ECMWF which are considered very high quality. This reveals good agreement between model and observations, albeit the model misses localized centers of wave activity if model resolution is too low.
Kathrin Baumgarten, Michael Gerding, Gerd Baumgarten, and Franz-Josef Lübken
Atmos. Chem. Phys., 18, 371–384, https://doi.org/10.5194/acp-18-371-2018, https://doi.org/10.5194/acp-18-371-2018, 2018
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Gravity waves (GWs) as well as solar tides are a key driving mechanism for the circulation in the Earth's atmosphere. The temporal variation of these waves is studied using a record long 10-day continuous Rayleigh–Mie–Raman lidar sounding at midlatitudes. This data set shows a large variability of these waves on timescales of a few days and therefore provides new insights into wave intermittency phenomena, which can help to improve model simulations.
Konstantinos S. Kalogerakis, Daniel Matsiev, Philip C. Cosby, James A. Dodd, Stefano Falcinelli, Jonas Hedin, Alexander A. Kutepov, Stefan Noll, Peter A. Panka, Constantin Romanescu, and Jérôme E. Thiebaud
Ann. Geophys., 36, 13–24, https://doi.org/10.5194/angeo-36-13-2018, https://doi.org/10.5194/angeo-36-13-2018, 2018
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The question of whether mesospheric rotational population distributions of vibrationally excited OH are in equilibrium with the local kinetic temperature has been debated over several decades. We examine the relationship of multi-quantum relaxation pathways with the behavior exhibited by OH(v) rotational population distributions and find that the effective rotational temperatures of mesospheric OH(v) deviate from local thermodynamic equilibrium for all observed vibrational levels.
Isabell Krisch, Peter Preusse, Jörn Ungermann, Andreas Dörnbrack, Stephen D. Eckermann, Manfred Ern, Felix Friedl-Vallon, Martin Kaufmann, Hermann Oelhaf, Markus Rapp, Cornelia Strube, and Martin Riese
Atmos. Chem. Phys., 17, 14937–14953, https://doi.org/10.5194/acp-17-14937-2017, https://doi.org/10.5194/acp-17-14937-2017, 2017
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Using the infrared limb imager GLORIA, the 3-D structure of mesoscale gravity waves in the lower stratosphere was measured for the first time, allowing for a complete 3-D characterization of the waves. This enables the precise determination of the sources of the waves in the mountain regions of Iceland with backward ray tracing. Forward ray tracing shows oblique propagation, an effect generally neglected in global atmospheric models.
Romy Heller, Christiane Voigt, Stuart Beaton, Andreas Dörnbrack, Andreas Giez, Stefan Kaufmann, Christian Mallaun, Hans Schlager, Johannes Wagner, Kate Young, and Markus Rapp
Atmos. Chem. Phys., 17, 14853–14869, https://doi.org/10.5194/acp-17-14853-2017, https://doi.org/10.5194/acp-17-14853-2017, 2017
Jens Hildebrand, Gerd Baumgarten, Jens Fiedler, and Franz-Josef Lübken
Atmos. Chem. Phys., 17, 13345–13359, https://doi.org/10.5194/acp-17-13345-2017, https://doi.org/10.5194/acp-17-13345-2017, 2017
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We present altitude profiles of winds and temperatures in the Arctic strato- and mesosphere obtained during three Januaries. The data show large year-to-year variations. We compare the observations to model data. For monthly mean profiles we find good agreement below 55 km altitude but also differences of up to 20 K and 20 m s-1 above. The fluctuations during single nights indicate gravity waves. The kinetic energy of such waves is typically 5 to 10 times larger than their potential energy.
Heiner Asmus, Tristan Staszak, Boris Strelnikov, Franz-Josef Lübken, Martin Friedrich, and Markus Rapp
Ann. Geophys., 35, 979–998, https://doi.org/10.5194/angeo-35-979-2017, https://doi.org/10.5194/angeo-35-979-2017, 2017
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This work sheds new light on the size distribution of dust grains of meteoric origin in the mesosphere and lower thermosphere region using rocket-borne instrumentation. We found that a large number of very small (~ 0.5 nm) particles are charged and therefore have a significant influence on the charge balance of the lower ionosphere.
Andreas Schneider, Johannes Wagner, Jens Faber, Michael Gerding, and Franz-Josef Lübken
Atmos. Chem. Phys., 17, 7941–7954, https://doi.org/10.5194/acp-17-7941-2017, https://doi.org/10.5194/acp-17-7941-2017, 2017
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Wave breaking is studied with a combination of high-resolution turbulence observations with the balloon-borne instrument LITOS and mesoscale simulations with the WRF model. A relation between observed turbulent energy dissipation rates and the occurrence of wave patterns in modelled vertical winds is found, which is interpreted as the effect of wave saturation. The change of stability plays less of a role for mean dissipation for the flights examined.
Yunxia Yuan, Nickolay Ivchenko, Gunnar Tibert, Marin Stanev, Jonas Hedin, and Jörg Gumbel
Atmos. Meas. Tech. Discuss., https://doi.org/10.5194/amt-2017-91, https://doi.org/10.5194/amt-2017-91, 2017
Revised manuscript has not been submitted
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The paper presents a method to determine altitude profile of atmospheric density, temperature and wind by means of analysing the reconstructed trajectory of a rigid falling sphere released from a sounding rocket. The trajectory reconstruction is achieved by post-flight analysis of GPS raw data gathered in the sphere. A comparison of the results with independent measurements is presented, with good agreement of the falling sphere results with other sources in the stratosphere.
Boris Strelnikov, Artur Szewczyk, Irina Strelnikova, Ralph Latteck, Gerd Baumgarten, Franz-Josef Lübken, Markus Rapp, Stefanos Fasoulas, Stefan Löhle, Martin Eberhart, Ulf-Peter Hoppe, Tim Dunker, Martin Friedrich, Jonas Hedin, Mikhail Khaplanov, Jörg Gumbel, and Aroh Barjatya
Ann. Geophys., 35, 547–565, https://doi.org/10.5194/angeo-35-547-2017, https://doi.org/10.5194/angeo-35-547-2017, 2017
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The WADIS sounding rocket mission utilized multi-point turbulence measurements in the mesosphere by different techniques, i.e., with ionization gauges carried by rockets and ground-based MAARSY and EISCAT radars. Results show that turbulence energy dissipation rates oscillate in space and time with amplitude of up to 2 orders of magnitude. Spatial oscillations show the same wavelengths as atmospheric gravity waves. Temporal variability reveals periods of atmospheric tides and gravity waves.
Johannes Wagner, Andreas Dörnbrack, Markus Rapp, Sonja Gisinger, Benedikt Ehard, Martina Bramberger, Benjamin Witschas, Fernando Chouza, Stephan Rahm, Christian Mallaun, Gerd Baumgarten, and Peter Hoor
Atmos. Chem. Phys., 17, 4031–4052, https://doi.org/10.5194/acp-17-4031-2017, https://doi.org/10.5194/acp-17-4031-2017, 2017
Qiang Li, Markus Rapp, Anne Schrön, Andreas Schneider, and Gunter Stober
Ann. Geophys., 34, 1209–1229, https://doi.org/10.5194/angeo-34-1209-2016, https://doi.org/10.5194/angeo-34-1209-2016, 2016
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Turbulence is an essential process in the atmosphere and ocean. Clear-air turbulence is a well-known threat for the safety of aviation. Using a powerful MST radar, we detected turbulence and compared it with the results from radiosondes. The correlation between turbulence and background conditions, e.g., Richardson number and wind shears, is determined. There is a nearly negative correlation between turbulence and Richardson number independent of the length scale over which it was calculated.
Franz-Josef Lübken, Gerd Baumgarten, Jens Hildebrand, and Francis J. Schmidlin
Atmos. Meas. Tech., 9, 3911–3919, https://doi.org/10.5194/amt-9-3911-2016, https://doi.org/10.5194/amt-9-3911-2016, 2016
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Wind measurements in the middle atmosphere (MA) are crucial to our understanding of atmospheric processes. We have recently developed a new laser-based method to measure winds called DoRIS (Doppler Rayleigh Iodine Spectrometer) which is the only technique to monitor winds in the middle atmosphere quasi-continuously. We
compare our measurements with rocket-borne measurements and find excellent
agreement above 30 km. DoRIS can now be considered as a validated method to measure winds in the MA.
Michael Gerding, Maren Kopp, Josef Höffner, Kathrin Baumgarten, and Franz-Josef Lübken
Atmos. Meas. Tech., 9, 3707–3715, https://doi.org/10.5194/amt-9-3707-2016, https://doi.org/10.5194/amt-9-3707-2016, 2016
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Temperature soundings by lidar are an important tool for the understanding of the middle atmosphere, including gravity waves and tides. Though, mesospheric lidar soundings at daytime are rare. We describe a daylight-capable RMR lidar with optical bandwidths in the range of the Doppler broadened laser backscatter. We account for the systematic temperature error induced by the optical filter, and present examples of daylight-independent temperature sounding as well as tidal analysis.
Carsten Baumann, Markus Rapp, and Antti Kero
Ann. Geophys., 34, 573–580, https://doi.org/10.5194/angeo-34-573-2016, https://doi.org/10.5194/angeo-34-573-2016, 2016
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Meteor smoke particles (MSPs), originating from evaporated meteoric matter at 60–110 km altitude, are present in the whole atmosphere including polar regions. As electron precipitation is present at high latitudes, these MSPs are bombarded by energetic electrons. The energetic electrons can enter the MSPs and excite secondary electrons. That can lead to a change of the charge state of these MSPs. The study finds that other charging processes, e.g., electron attachment, are more important.
J. Kiliani, G. Baumgarten, F.-J. Lübken, and U. Berger
Atmos. Chem. Phys., 15, 12897–12907, https://doi.org/10.5194/acp-15-12897-2015, https://doi.org/10.5194/acp-15-12897-2015, 2015
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For the first time the shape of noctilucent cloud particles is analyzed with a 3-D Lagrangian model. Three-color lidar measurements are compared directly to optical modeling of NLC simulations with non-spherical shapes: a mix of elongated and flattened cylindrical ice particles consistent with measurements. Comparison is best if flattened particles form a majority, with mean axis ratio around 2.8. NLCs from cylindrical particles are slightly brighter and consist of fewer but larger ice particle.
B. Ehard, B. Kaifler, N. Kaifler, and M. Rapp
Atmos. Meas. Tech., 8, 4645–4655, https://doi.org/10.5194/amt-8-4645-2015, https://doi.org/10.5194/amt-8-4645-2015, 2015
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We evalute four methods currently used for gravity wave extraction from lidar temperature measurements. The spectral response of these methods is determined with the help of synthetic temperature perturbations. Afterwards, the methods are applied to lidar temperature measurements over New Zealand for further evaluation of the four algorithms. Based on the results two methods are recommended for gravity wave extraction.
M. Eberhart, S. Löhle, A. Steinbeck, T. Binder, and S. Fasoulas
Atmos. Meas. Tech., 8, 3701–3714, https://doi.org/10.5194/amt-8-3701-2015, https://doi.org/10.5194/amt-8-3701-2015, 2015
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In this paper we report on the first-time use of solid electrolyte sensors for selectively measuring atomic oxygen aboard sounding rockets. Together with our second system based on catalytic probes they were part of the WADIS-1 campaign in northern Norway and retrieved density profiles in Earth's middle atmosphere. Sensor data have a high spatial resolution and show small-scall density variations. Profiles are compared to literature data and previous flight results.
M. Placke, P. Hoffmann, and M. Rapp
Ann. Geophys., 33, 1091–1096, https://doi.org/10.5194/angeo-33-1091-2015, https://doi.org/10.5194/angeo-33-1091-2015, 2015
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Imposed momentum from mesospheric breaking gravity waves (GWs) is conserved by a balance between vertical divergence of GW momentum flux and Coriolis acceleration of the mean meridional wind. We present the first experimental verification of the momentum balance from the Saura MF radar at 69°N. For contributions from GWs only this balance is fulfilled between 70 and 100km during summer when GWs dominate the mesospheric dynamics, but it does not exist in winter due to planetary wave impacts.
O. M. Christensen, P. Eriksson, J. Urban, D. Murtagh, K. Hultgren, and J. Gumbel
Atmos. Meas. Tech., 8, 1981–1999, https://doi.org/10.5194/amt-8-1981-2015, https://doi.org/10.5194/amt-8-1981-2015, 2015
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Polar mesospheric clouds are clouds that form in the summer polar mesopause, 80km above the surface. In this study we present new measurements by the Odin satellite, which are able to determine water vapour, temperature and cloud coverage with a high resolution and a large geographical coverage. Using these data we can see structures in the clouds and background atmosphere that have not been detectable by previous measurements.
A. Schneider, M. Gerding, and F.-J. Lübken
Atmos. Chem. Phys., 15, 2159–2166, https://doi.org/10.5194/acp-15-2159-2015, https://doi.org/10.5194/acp-15-2159-2015, 2015
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Stratospheric turbulence is essential for the atmospheric energy budget. We compare in situ observations with our LITOS method based on spectral analysis of mm-scale wind fluctuations with the Thorpe method applied to standard radiosondes. Energy dissipations rates from both methods differ by up to 3 orders of magnitude. Nevertheless, mean values are in good agreement. We present case studies on both methods and examine the applicability of the Thorpe method for calculation of dissipation rates.
V. Matthias, T. G. Shepherd, P. Hoffmann, and M. Rapp
Ann. Geophys., 33, 199–206, https://doi.org/10.5194/angeo-33-199-2015, https://doi.org/10.5194/angeo-33-199-2015, 2015
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A vertical coupling process in the northern high-latitude middle atmosphere has been identified during the equinox transitions, which we call the “hiccup” and which acts like a “mini sudden stratospheric warming (SSW)”. We study the average characteristics of the hiccup based on a composite analysis using a nudged model. A comparison of the average characteristics of hiccups and SSWs shows both similarities and differences between the two vertical coupling processes.
B. Ehard, P. Achtert, and J. Gumbel
Ann. Geophys., 32, 1395–1405, https://doi.org/10.5194/angeo-32-1395-2014, https://doi.org/10.5194/angeo-32-1395-2014, 2014
H. Wilms, M. Rapp, P. Hoffmann, J. Fiedler, and G. Baumgarten
Atmos. Chem. Phys., 13, 11951–11963, https://doi.org/10.5194/acp-13-11951-2013, https://doi.org/10.5194/acp-13-11951-2013, 2013
N. Kaifler, G. Baumgarten, J. Fiedler, and F.-J. Lübken
Atmos. Chem. Phys., 13, 11757–11768, https://doi.org/10.5194/acp-13-11757-2013, https://doi.org/10.5194/acp-13-11757-2013, 2013
C. Baumann, M. Rapp, A. Kero, and C.-F. Enell
Ann. Geophys., 31, 2049–2062, https://doi.org/10.5194/angeo-31-2049-2013, https://doi.org/10.5194/angeo-31-2049-2013, 2013
G. Stober, S. Sommer, M. Rapp, and R. Latteck
Atmos. Meas. Tech., 6, 2893–2905, https://doi.org/10.5194/amt-6-2893-2013, https://doi.org/10.5194/amt-6-2893-2013, 2013
V. Matthias, P. Hoffmann, A. Manson, C. Meek, G. Stober, P. Brown, and M. Rapp
Ann. Geophys., 31, 1397–1415, https://doi.org/10.5194/angeo-31-1397-2013, https://doi.org/10.5194/angeo-31-1397-2013, 2013
A. Szewczyk, B. Strelnikov, M. Rapp, I. Strelnikova, G. Baumgarten, N. Kaifler, T. Dunker, and U.-P. Hoppe
Ann. Geophys., 31, 775–785, https://doi.org/10.5194/angeo-31-775-2013, https://doi.org/10.5194/angeo-31-775-2013, 2013
G. Stober, C. Schult, C. Baumann, R. Latteck, and M. Rapp
Ann. Geophys., 31, 473–487, https://doi.org/10.5194/angeo-31-473-2013, https://doi.org/10.5194/angeo-31-473-2013, 2013
I. Strelnikova and M. Rapp
Ann. Geophys., 31, 359–375, https://doi.org/10.5194/angeo-31-359-2013, https://doi.org/10.5194/angeo-31-359-2013, 2013
P. Achtert, M. Khaplanov, F. Khosrawi, and J. Gumbel
Atmos. Meas. Tech., 6, 91–98, https://doi.org/10.5194/amt-6-91-2013, https://doi.org/10.5194/amt-6-91-2013, 2013
M. Rapp, J. M. C. Plane, B. Strelnikov, G. Stober, S. Ernst, J. Hedin, M. Friedrich, and U.-P. Hoppe
Ann. Geophys., 30, 1661–1673, https://doi.org/10.5194/angeo-30-1661-2012, https://doi.org/10.5194/angeo-30-1661-2012, 2012
Related subject area
Subject: Gases | Technique: In Situ Measurement | Topic: Instruments and Platforms
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Daniel Furuta, Bruce Wilson, Albert A. Presto, and Jiayu Li
Atmos. Meas. Tech., 17, 2103–2121, https://doi.org/10.5194/amt-17-2103-2024, https://doi.org/10.5194/amt-17-2103-2024, 2024
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Methane is an important driver of climate change and is challenging to inexpensively sense in low atmospheric concentrations. We developed a low-cost sensor to monitor methane and tested it in indoor and outdoor settings. Our device shows promise for monitoring low levels of methane. We characterize its limitations and suggest future research directions for further development.
Audrey J. Dang, Nathan M. Kreisberg, Tyler L. Cargill, Jhao-Hong Chen, Sydney Hornitschek, Remy Hutheesing, Jay R. Turner, and Brent J. Williams
Atmos. Meas. Tech., 17, 2067–2087, https://doi.org/10.5194/amt-17-2067-2024, https://doi.org/10.5194/amt-17-2067-2024, 2024
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The Multichannel Organics In situ enviRonmental Analyzer (MOIRA) is a new instrument for measuring speciated volatile organic compounds (VOCs) in the air and has been developed for mapping concentrations from a hybrid car. MOIRA is characterized in the lab and pilot field studies of indoor air in a single-family residence and outdoor air during a mobile deployment. Future applications include indoor, outdoor, and lab measurements to grasp the impact of VOCs on air quality, health, and climate.
Asher P. Mouat, Zelda A. Siegel, and Jennifer Kaiser
Atmos. Meas. Tech., 17, 1979–1994, https://doi.org/10.5194/amt-17-1979-2024, https://doi.org/10.5194/amt-17-1979-2024, 2024
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Three fast-measurement formaldehyde monitors were deployed at two field sites in Atlanta, GA, over 1 year. Four different zeroing methods were tested to develop an optimal field setup as well as procedures for instrument calibration. Observations agreed well after calibration but were much higher compared to the TO-11A monitoring method, which is the golden standard. Historical HCHO concentrations were compared with measurements in this work, showing a 22 % reduction in midday HCHO since 1999.
Da Yang, Margarita Reza, Roy Mauldin, Rainer Volkamer, and Suresh Dhaniyala
Atmos. Meas. Tech., 17, 1463–1474, https://doi.org/10.5194/amt-17-1463-2024, https://doi.org/10.5194/amt-17-1463-2024, 2024
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This paper evaluates the performance of an aircraft gas inlet. Here, we use computational fluid dynamics (CFD) and experiments to demonstrate the role of turbulence in determining sampling performance of a gas inlet and identify ideal conditions for inlet operation to minimize gas loss. Experiments conducted in a high-speed wind tunnel under near-aircraft speeds validated numerical results. We believe that the results obtained from this work will greatly inform future gas inlet studies.
Reena Macagga, Michael Asante, Geoffroy Sossa, Danica Antonijević, Maren Dubbert, and Mathias Hoffmann
Atmos. Meas. Tech., 17, 1317–1332, https://doi.org/10.5194/amt-17-1317-2024, https://doi.org/10.5194/amt-17-1317-2024, 2024
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Using only low-cost microcontrollers and sensors, we constructed a measurement device to accurately and precisely obtain atmospheric carbon dioxide and water fluxes. The device was tested against known concentration increases and high-cost, commercial sensors during a laboratory and field experiment. We additionally tested the device over a longer period in a field study in Ghana during which the net ecosystem carbon balance and water use efficiency of maize cultivation were studied.
Matthew M. Coggon, Chelsea E. Stockwell, Megan S. Claflin, Eva Y. Pfannerstill, Lu Xu, Jessica B. Gilman, Julia Marcantonio, Cong Cao, Kelvin Bates, Georgios I. Gkatzelis, Aaron Lamplugh, Erin F. Katz, Caleb Arata, Eric C. Apel, Rebecca S. Hornbrook, Felix Piel, Francesca Majluf, Donald R. Blake, Armin Wisthaler, Manjula Canagaratna, Brian M. Lerner, Allen H. Goldstein, John E. Mak, and Carsten Warneke
Atmos. Meas. Tech., 17, 801–825, https://doi.org/10.5194/amt-17-801-2024, https://doi.org/10.5194/amt-17-801-2024, 2024
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Mass spectrometry is a tool commonly used to measure air pollutants. This study evaluates measurement artifacts produced in the proton-transfer-reaction mass spectrometer. We provide methods to correct these biases and better measure compounds that degrade air quality.
Tianran Han, Conghui Xie, Yayong Liu, Yanrong Yang, Yuheng Zhang, Yufei Huang, Xiangyu Gao, Xiaohua Zhang, Fangmin Bao, and Shao-Meng Li
Atmos. Meas. Tech., 17, 677–691, https://doi.org/10.5194/amt-17-677-2024, https://doi.org/10.5194/amt-17-677-2024, 2024
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This study reported an integrated UAV measurement platform for GHG monitoring and its application for emission quantification from a coking plant. The key element of this system is a newly designed air sampler, consisting of a 150 m long tube with remote-controlled time stamping. When comparing the top-down results to those derived from the bottom-up inventory method, the present findings indicate that the use of IPCC emission factors for emission calculations can lead to overestimation.
Yuening Li, Faqiang Zhan, Yushan Su, Ying Duan Lei, Chubashini Shunthirasingham, Zilin Zhou, Jonathan P. D. Abbatt, Hayley Hung, and Frank Wania
Atmos. Meas. Tech., 17, 715–729, https://doi.org/10.5194/amt-17-715-2024, https://doi.org/10.5194/amt-17-715-2024, 2024
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A simple device for sampling gases from the atmosphere without the help of pumps was calibrated for an important group of hazardous air pollutants called polycyclic aromatic compounds (PACs). While the sampler appeared to perform well when used for relatively short periods of up to several months, some PACs were lost from the sampler during longer deployments. Sampling rates that can be used to quantitatively interpret the quantities of PACs taken up in the device have been derived.
Roger Curcoll, Claudia Grossi, Stefan Röttger, and Arturo Vargas
EGUsphere, https://doi.org/10.5194/egusphere-2023-2680, https://doi.org/10.5194/egusphere-2023-2680, 2023
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The new version of the Atmospheric Radon MONitor (ARMON) is presented. The monitor efficiency and its linearity over a wide spam of radon concentration activities is evaluated and tested, with a complete budget analysis of the total uncertainty. Results obtained supports the applicability of the ARMON to measure low-level radon activity concentration with an uncertainty lower than 10 % and to be used as transfer standard to calibrate secondary atmospheric radon monitors.
Jiaxin Li, Kunpeng Zang, Yi Lin, Yuanyuan Chen, Shuo Liu, Shanshan Qiu, Kai Jiang, Xuemei Qing, Haoyu Xiong, Haixiang Hong, Shuangxi Fang, Honghui Xu, and Yujun Jiang
Atmos. Meas. Tech., 16, 4757–4768, https://doi.org/10.5194/amt-16-4757-2023, https://doi.org/10.5194/amt-16-4757-2023, 2023
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Based on observed data of CO2 and CH4 and meteorological parameters over the Yellow Sea in November 2012 and June 2013, a data process and quality control method was optimized and established to filter the data influenced by multiple factors. Spatial and seasonal variations in CO2 and CH4 mixing ratios were mainly controlled by the East Asian Monsoon, while the influence of air–sea exchange was slight.
Zaneta Hamryszczak, Antonia Hartmann, Dirk Dienhart, Sascha Hafermann, Bettina Brendel, Rainer Königstedt, Uwe Parchatka, Jos Lelieveld, and Horst Fischer
Atmos. Meas. Tech., 16, 4741–4756, https://doi.org/10.5194/amt-16-4741-2023, https://doi.org/10.5194/amt-16-4741-2023, 2023
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Hydroperoxide measurements improve the understanding of atmospheric oxidation processes. We introduce an instrumental setup for airborne measurements. The aim of the work is the characterization of the measurement method with emphasis on interferences impacting instrumental uncertainty. Technical and physical challenges do not critically impact the instrumental performance. The instrument resolves dynamic processes, such as convective transport, as shown based on the CAFE-Brazil campaign.
James F. Hurley, Alejandra Caceres, Deborah F. McGlynn, Mary E. Tovillo, Suzanne Pinar, Roger Schürch, Ksenia Onufrieva, and Gabriel Isaacman-VanWertz
Atmos. Meas. Tech., 16, 4681–4692, https://doi.org/10.5194/amt-16-4681-2023, https://doi.org/10.5194/amt-16-4681-2023, 2023
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Volatile organic compounds (VOCs) have a wide range of sources and impacts on environments and human health that make them spatially, temporally, and chemically varied. Current methods lack the ability to collect samples in ways that provide spatial and chemical resolution without complex, costly instrumentation. We describe and validate a low-cost, portable VOC sampler and demonstrate its utility in collecting distributed coordinated samples.
Simone Brunamonti, Manuel Graf, Tobias Bühlmann, Céline Pascale, Ivan Ilak, Lukas Emmenegger, and Béla Tuzson
Atmos. Meas. Tech., 16, 4391–4407, https://doi.org/10.5194/amt-16-4391-2023, https://doi.org/10.5194/amt-16-4391-2023, 2023
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The abundance of water vapor (H2O) in the upper atmosphere has a significant impact on the rate of global warming. We developed a new lightweight spectrometer (ALBATROSS) for H2O measurements aboard meteorological balloons. Here, we assess the accuracy and precision of ALBATROSS using metrology-grade reference gases. The results demonstrate the exceptional potential of mid-infrared laser absorption spectroscopy as a new reference method for in situ measurements of H2O in the upper atmosphere.
Josie K. Radtke, Benjamin N. Kies, Whitney A. Mottishaw, Sydney M. Zeuli, Aidan T. H. Voon, Kelly L. Koerber, Grant W. Petty, Michael Vermeuel, Timothy H. Bertram, Ankur R. Desai, Joseph P. Hupy, R. Bradley Pierce, Timothy J. Wagner, and Patricia A. Cleary
Atmos. Meas. Tech. Discuss., https://doi.org/10.5194/amt-2023-143, https://doi.org/10.5194/amt-2023-143, 2023
Revised manuscript accepted for AMT
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This research focused on impact of Chicago pollution plumes on a shoreline area in Kenosha, WI to address the regional issue of high ozone concentrations which get confined within marine air masses over Lake Michigan and move on shore during lake breezes. This manuscript describes the unmanned aerial systems (UAS) observations near the Lake Michigan shoreline that show layers of ozone within this marine air.
Chen-Wei Liang and Chang-Hung Shen
Atmos. Meas. Tech. Discuss., https://doi.org/10.5194/amt-2023-162, https://doi.org/10.5194/amt-2023-162, 2023
Revised manuscript accepted for AMT
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In the present study, a UAV platform with sensing and sampling systems was developed for 3D air pollutant concentration measurements. The sensing system of this platform contains multiple microsensors and IoT technologies for obtaining the real-time 3D distributions of critical air pollutants. The sampling system contains gas sampling sets, and a 1-L Tedlar bag instead of a canister for the 3D measurement of VOC concentrations in accordance with the TO-15 method of the US EPA.
Zihan Zhu, Javier Gonzalez-Rocha, Yifan Ding, Isis Frausto-Vicencio, Sajjan Heerah, Akula Venkatram, Manvendra Dubey, Don Collins, and Francesca Hopkins
EGUsphere, https://doi.org/10.5194/egusphere-2023-1527, https://doi.org/10.5194/egusphere-2023-1527, 2023
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Increases in agriculture, oil and gas, and waste management activities have contributed to the growth of atmospheric methane levels and climate warming. In this manuscript, we explore the use of small uncrewed aircraft systems (sUAS) and Aircore technology to detect and quantify methane emissions. Results from field experiments demonstrate that sUAS and Aircore technology can be effective for detecting and quantifying methane emissions in near real-time.
Roubina Papaconstantinou, Marios Demosthenous, Spyros Bezantakos, Neoclis Hadjigeorgiou, Marinos Costi, Melina Stylianou, Elli Symeou, Chrysanthos Savvides, and George Biskos
Atmos. Meas. Tech., 16, 3313–3329, https://doi.org/10.5194/amt-16-3313-2023, https://doi.org/10.5194/amt-16-3313-2023, 2023
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In this paper, we investigate the performance of low-cost electrochemical gas sensors. We carried out yearlong measurements at a traffic air quality monitoring station, where the low-cost sensors were collocated with reference instruments and exposed to highly variable environmental conditions with extremely high temperatures and low relative humidity (RH). Sensors provide measurements that exhibit increasing errors and decreasing correlations as temperature increases and RH decreases.
Jianghanyang Li, Bianca C. Baier, Fred Moore, Tim Newberger, Sonja Wolter, Jack Higgs, Geoff Dutton, Eric Hintsa, Bradley Hall, and Colm Sweeney
Atmos. Meas. Tech., 16, 2851–2863, https://doi.org/10.5194/amt-16-2851-2023, https://doi.org/10.5194/amt-16-2851-2023, 2023
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Monitoring a suite of trace gases in the stratosphere will help us better understand the stratospheric circulation and its impact on the earth's radiation balance. However, such measurements are rare and usually expensive. We developed an instrument that can measure stratospheric trace gases using a low-cost sampling platform (AirCore). The results showed expected agreement with aircraft measurements, demonstrating this technique provides a low-cost and robust way to observe the stratosphere.
Tara I. Yacovitch, Christoph Dyroff, Joseph R. Roscioli, Conner Daube, J. Barry McManus, and Scott C. Herndon
Atmos. Meas. Tech., 16, 1915–1921, https://doi.org/10.5194/amt-16-1915-2023, https://doi.org/10.5194/amt-16-1915-2023, 2023
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Ethylene oxide is a toxic, carcinogenic compound used in the medical and bulk sterilization industry. Here we describe a precise and fast laser-based ethylene oxide monitor. We report months-long concentrations at a Massachusetts site, and we show how they suggest a potential emission source 35 km away. This source, and another, is confirmed by driving the instrument downwind of the sites, where concentrations were tens to tens of thousands of times greater than background levels.
Tatsumi Nakano and Takashi Morofuji
Atmos. Meas. Tech., 16, 1583–1595, https://doi.org/10.5194/amt-16-1583-2023, https://doi.org/10.5194/amt-16-1583-2023, 2023
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We have developed a system that can automatically measure the pump efficiency of the ECC-type ozonesonde. Operational measurement for 13 years by this system revealed that the efficiency fluctuates in each and slightly increases over time. Those can affect the estimation of total ozone amount by up to 4 %. This result indicates that it is necessary to understand the tendency of the pump correction factor of each ozonesonde in order to detect the actual atmospheric change with high accuracy.
Benjamin Birner, Eric Morgan, and Ralph F. Keeling
Atmos. Meas. Tech., 16, 1551–1561, https://doi.org/10.5194/amt-16-1551-2023, https://doi.org/10.5194/amt-16-1551-2023, 2023
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Atmospheric variations of helium (He) and CO2 are strongly linked due to the co-release of both gases from natural-gas burning. This implies that atmospheric He measurements may be a potentially powerful tool for verifying reported anthropogenic natural-gas usage. Here, we present the development and initial results of a novel measurement system of atmospheric He that paves the way for establishing a global monitoring network in the future.
John W. Halfacre, Jordan Stewart, Scott C. Herndon, Joseph R. Roscioli, Christoph Dyroff, Tara I. Yacovitch, Michael Flynn, Stephen J. Andrews, Steven S. Brown, Patrick R. Veres, and Pete M. Edwards
Atmos. Meas. Tech., 16, 1407–1429, https://doi.org/10.5194/amt-16-1407-2023, https://doi.org/10.5194/amt-16-1407-2023, 2023
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This study details a new sampling method for the optical detection of hydrogen chloride (HCl). HCl is an important atmospheric reservoir for chlorine atoms, which can affect nitrogen oxide cycling and the lifetimes of volatile organic compounds and ozone. However, HCl has a high affinity for interacting with surfaces, thereby preventing fast, quantitative measurements. The sampling technique in this study minimizes these surface interactions and provides a high-quality measurement of HCl.
Henning Finkenzeller, Denis Pöhler, Martin Horbanski, Johannes Lampel, and Ulrich Platt
Atmos. Meas. Tech., 16, 1343–1356, https://doi.org/10.5194/amt-16-1343-2023, https://doi.org/10.5194/amt-16-1343-2023, 2023
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Optical resonators enhance the light path in compact instruments, thereby improving their sensitivity. Determining the established path length in the instrument is a prerequisite for the accurate determination of trace gas concentrations but can be a significant complication in the use of such resonators. Here we show two calibration techniques which are relatively simple and free of consumables but still provide accurate calibrations. This facilitates the use of optical resonators.
Andrew W. Seidl, Harald Sodemann, and Hans Christian Steen-Larsen
Atmos. Meas. Tech., 16, 769–790, https://doi.org/10.5194/amt-16-769-2023, https://doi.org/10.5194/amt-16-769-2023, 2023
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It is challenging to make field measurements of stable water isotopes in the Arctic. To this end, we present a modular stable-water-isotope analyzer profiling system. The system operated for a 2-week field campaign on Svalbard during the Arctic winter. We evaluate the system’s performance and analyze any potential impact that the field conditions might have had on the isotopic measurements and the system's ability to resolve isotope gradients in the lowermost layer of the atmosphere.
Daan Swart, Jun Zhang, Shelley van der Graaf, Susanna Rutledge-Jonker, Arjan Hensen, Stijn Berkhout, Pascal Wintjen, René van der Hoff, Marty Haaima, Arnoud Frumau, Pim van den Bulk, Ruben Schulte, Margreet van Zanten, and Thomas van Goethem
Atmos. Meas. Tech., 16, 529–546, https://doi.org/10.5194/amt-16-529-2023, https://doi.org/10.5194/amt-16-529-2023, 2023
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During a 5-week comparison campaign, we tested two set-ups to measure half hourly ammonia fluxes. The eddy covariance and flux gradient systems showed very similar results when the upwind terrain was both homogeneous and free of obstacles. We discuss the technical performance and practical limitations of both systems. Measurements from these instruments can facilitate the study of processes behind ammonia deposition, an important contributor to eutrophication and acidificationin natural areas.
Suding Yang, Xin Li, Limin Zeng, Xuena Yu, Ying Liu, Sihua Lu, Xiaofeng Huang, Dongmei Zhang, Haibin Xu, Shuchen Lin, Hefan Liu, Miao Feng, Danlin Song, Qinwen Tan, Jinhui Cui, Lifan Wang, Ying Chen, Wenjie Wang, Haijiong Sun, Mengdi Song, Liuwei Kong, Yi Liu, Linhui Wei, Xianwu Zhu, and Yuanhang Zhang
Atmos. Meas. Tech., 16, 501–512, https://doi.org/10.5194/amt-16-501-2023, https://doi.org/10.5194/amt-16-501-2023, 2023
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Vertical observation of volatile organic compounds (VOCs) is essential to study the spatial distribution and evolution patterns of VOCs in the planetary boundary layer (PBL). This paper describes multi-channel whole-air sampling equipment onboard an unmanned aerial vehicle (UAV) for near-continuous VOC vertical observation. Vertical profiles of VOCs and trace gases during the evolution of the PBL in south-western China have been successfully obtained by deploying the newly developed UAV system.
Tobias Schuldt, Georgios I. Gkatzelis, Christian Wesolek, Franz Rohrer, Benjamin Winter, Thomas A. J. Kuhlbusch, Astrid Kiendler-Scharr, and Ralf Tillmann
Atmos. Meas. Tech., 16, 373–386, https://doi.org/10.5194/amt-16-373-2023, https://doi.org/10.5194/amt-16-373-2023, 2023
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We report in situ measurements of air pollutant concentrations within the planetary boundary layer on board a Zeppelin NT in Germany. We highlight the in-flight evaluation of electrochemical sensors that were installed inside a hatch box located on the bottom of the Zeppelin. Results from this work emphasize the potential of these sensors for other in situ airborne applications, e.g., on board unmanned aerial vehicles (UAVs).
Leigh S. Fleming, Andrew C. Manning, Penelope A. Pickers, Grant L. Forster, and Alex J. Etchells
Atmos. Meas. Tech., 16, 387–401, https://doi.org/10.5194/amt-16-387-2023, https://doi.org/10.5194/amt-16-387-2023, 2023
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Measurements of atmospheric O2 can help constrain the carbon cycle processes and quantify fossil fuel CO2 emissions; however, measurement of atmospheric O2 is very challenging, and existing analysers are complex systems to build and maintain. We have tested a new O2 analyser (Picarro Inc. G2207-i) in the laboratory and at Weybourne Atmospheric Observatory. We have found that the G2207-i does not perform as well as an existing O2 analyser from Sable Systems Inc.
Siegfried Schobesberger, Emma L. D'Ambro, Lejish Vettikkat, Ben H. Lee, Qiaoyun Peng, David M. Bell, John E. Shilling, Manish Shrivastava, Mikhail Pekour, Jerome Fast, and Joel A. Thornton
Atmos. Meas. Tech., 16, 247–271, https://doi.org/10.5194/amt-16-247-2023, https://doi.org/10.5194/amt-16-247-2023, 2023
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We present a new, highly sensitive technique for measuring atmospheric ammonia, an important trace gas that is emitted mainly by agriculture. We deployed the instrument on an aircraft during research flights over rural Oklahoma. Due to its fast response, we could analyze correlations with turbulent winds and calculate ammonia emissions from nearby areas at 1 to 2 km resolution. We observed high spatial variability and point sources that are not resolved in the US National Emissions Inventory.
Birger Bohn and Insa Lohse
Atmos. Meas. Tech., 16, 209–233, https://doi.org/10.5194/amt-16-209-2023, https://doi.org/10.5194/amt-16-209-2023, 2023
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Optical receivers for solar spectral actinic radiation are designed for angle-independent sensitivities within a hemisphere. Remaining imperfections can be compensated for by receiver-specific corrections based on laboratory characterizations and radiative transfer calculations of spectral radiance distributions. The corrections cover a wide range of realistic atmospheric conditions and were applied to ground-based and airborne measurements in a wavelength range 280–660 nm.
Teles C. Furlani, RenXi Ye, Jordan Stewart, Leigh R. Crilley, Peter M. Edwards, Tara F. Kahan, and Cora J. Young
Atmos. Meas. Tech., 16, 181–193, https://doi.org/10.5194/amt-16-181-2023, https://doi.org/10.5194/amt-16-181-2023, 2023
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This study describes a new technique to measure total gaseous chlorine, which is the sum of gas-phase chlorine-containing chemicals. The method converts any chlorine-containing molecule to hydrogen chloride that can be detected in real time using a cavity ring-down spectrometer. The new method was validated through laboratory experiments, as well as by making measurements of ambient outdoor air and indoor air during cleaning with a chlorine-based cleaner.
Anas Emad and Lukas Siebicke
Atmos. Meas. Tech., 16, 29–40, https://doi.org/10.5194/amt-16-29-2023, https://doi.org/10.5194/amt-16-29-2023, 2023
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The true eddy accumulation (TEA) method enables measuring atmospheric exchange with slow-response gas analyzers. TEA is formulated assuming ideal conditions with a zero mean vertical wind velocity during the averaging interval. This core assumption is rarely valid under field conditions. Here, we extend the TEA equation to accommodate nonideal conditions. The new equation allows constraining the systematic error term in the measured fluxes and the possibility to minimize or remove it.
Anas Emad and Lukas Siebicke
Atmos. Meas. Tech., 16, 41–55, https://doi.org/10.5194/amt-16-41-2023, https://doi.org/10.5194/amt-16-41-2023, 2023
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A new micrometeorological method to measure atmospheric exchange is proposed, and a prototype sampler is evaluated. The new method, called short-time eddy accumulation, is a variant of the eddy accumulation method, which is suited for use with slow gas analyzers. The new method enables adaptive time-varying accumulation intervals, which brings many advantages to flux measurements such as an improved dynamic range and the ability to run eddy accumulation in a continuous flow-through mode.
Jean-Louis Bonne, Ludovic Donnat, Grégory Albora, Jérémie Burgalat, Nicolas Chauvin, Delphine Combaz, Julien Cousin, Thomas Decarpenterie, Olivier Duclaux, Nicolas Dumelié, Nicolas Galas, Catherine Juery, Florian Parent, Florent Pineau, Abel Maunoury, Olivier Ventre, Marie-France Bénassy, and Lilian Joly
Atmos. Meas. Tech. Discuss., https://doi.org/10.5194/amt-2022-334, https://doi.org/10.5194/amt-2022-334, 2023
Revised manuscript accepted for AMT
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We present a top-down approach to quantify CO2 and CH4 emissions at the scale of an industrial site, based on a mass balance model relying on atmospheric concentrations measurements from a new sensor embarked on-board Unmanned Aircraft Vehicles (UAVs). We present a laboratory characterization of our sensor and a field validation of our quantification method, together with field application to the monitoring of two real-world offshore oil and gas platforms.
Lu Xu, Matthew M. Coggon, Chelsea E. Stockwell, Jessica B. Gilman, Michael A. Robinson, Martin Breitenlechner, Aaron Lamplugh, John D. Crounse, Paul O. Wennberg, J. Andrew Neuman, Gordon A. Novak, Patrick R. Veres, Steven S. Brown, and Carsten Warneke
Atmos. Meas. Tech., 15, 7353–7373, https://doi.org/10.5194/amt-15-7353-2022, https://doi.org/10.5194/amt-15-7353-2022, 2022
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We describe the development and operation of a chemical ionization mass spectrometer using an ammonium–water cluster (NH4+·H2O) as a reagent ion. NH4+·H2O is a highly versatile reagent ion for measurements of a wide range of oxygenated organic compounds. The major product ion is the cluster with NH4+ produced via ligand-switching reactions. The instrumental sensitivities of analytes depend on the binding energy of the analyte–NH4+ cluster; sensitivities can be estimated using voltage scanning.
Xiaorui Chen, Haichao Wang, Tianyu Zhai, Chunmeng Li, and Keding Lu
Atmos. Meas. Tech., 15, 7019–7037, https://doi.org/10.5194/amt-15-7019-2022, https://doi.org/10.5194/amt-15-7019-2022, 2022
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N2O5 is an important reservoir of atmospheric nitrogen, on whose interface reaction ambient particles can largely influence the fate of nitrogen oxides and air quality. In this study, we develop an approach to enable the reactions of N2O5 on ambient particles directly in a tube reactor, deriving the reaction rates with high accuracy by means of a chemistry model. Its successful application helps complement the data scarcity and to fill the knowledge gap between laboratory and field results.
Yubin Chen, Bin Yuan, Chaomin Wang, Sihang Wang, Xianjun He, Caihong Wu, Xin Song, Yibo Huangfu, Xiao-Bing Li, Yijia Liao, and Min Shao
Atmos. Meas. Tech., 15, 6935–6947, https://doi.org/10.5194/amt-15-6935-2022, https://doi.org/10.5194/amt-15-6935-2022, 2022
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In this study, we demonstrate that selective online measurements of cycloalkanes can be achieved using proton transfer reaction time-of-flight mass spectrometry with NO+ chemical ionization (NO+ PTR-ToF-MS), with fast response and low detection limits. Applications of this method in both urban air and emission sources will be shown.
Marsailidh M. Twigg, Augustinus J. C. Berkhout, Nicholas Cowan, Sabine Crunaire, Enrico Dammers, Volker Ebert, Vincent Gaudion, Marty Haaima, Christoph Häni, Lewis John, Matthew R. Jones, Bjorn Kamps, John Kentisbeer, Thomas Kupper, Sarah R. Leeson, Daiana Leuenberger, Nils O. B. Lüttschwager, Ulla Makkonen, Nicholas A. Martin, David Missler, Duncan Mounsor, Albrecht Neftel, Chad Nelson, Eiko Nemitz, Rutger Oudwater, Celine Pascale, Jean-Eudes Petit, Andrea Pogany, Nathalie Redon, Jörg Sintermann, Amy Stephens, Mark A. Sutton, Yuk S. Tang, Rens Zijlmans, Christine F. Braban, and Bernhard Niederhauser
Atmos. Meas. Tech., 15, 6755–6787, https://doi.org/10.5194/amt-15-6755-2022, https://doi.org/10.5194/amt-15-6755-2022, 2022
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Ammonia (NH3) gas in the atmosphere impacts the environment, human health, and, indirectly, climate. Historic NH3 monitoring was labour intensive, and the instruments were complicated. Over the last decade, there has been a rapid technology development, including “plug-and-play” instruments. This study is an extensive field comparison of the currently available technologies and provides evidence that for routine monitoring, standard operating protocols are required for datasets to be comparable.
Caroline C. Womack, Steven S. Brown, Steven J. Ciciora, Ru-Shan Gao, Richard J. McLaughlin, Michael A. Robinson, Yinon Rudich, and Rebecca A. Washenfelder
Atmos. Meas. Tech., 15, 6643–6652, https://doi.org/10.5194/amt-15-6643-2022, https://doi.org/10.5194/amt-15-6643-2022, 2022
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We present a new miniature instrument to measure nitrogen dioxide (NO2) using cavity-enhanced spectroscopy. NO2 contributes to the formation of pollutants such as ozone and particulate matter, and its concentration can vary widely near sources. We developed this lightweight (3.05 kg) low-power (<35 W) instrument to measure NO2 on uncrewed aircraft vehicles (UAVs) and demonstrate that it has the accuracy and precision needed for atmospheric field measurements.
Alexander Håland, Tomáš Mikoviny, Elisabeth Emilie Syse, and Armin Wisthaler
Atmos. Meas. Tech., 15, 6297–6307, https://doi.org/10.5194/amt-15-6297-2022, https://doi.org/10.5194/amt-15-6297-2022, 2022
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PTR-MS is widely used in atmospheric sciences for the detection of non-methane organic trace gases. The two most widely used types of PTR-MS instruments differ in their ion source and drift tube design. We herein present a new prototype PTR-MS instrument that hybridizes these designs and combines a conventional hollow cathode glow discharge ion source with a focusing ion–molecule reactor. We also show how this new instrument performs in detecting atmospheric amines.
Gustavo Britto Hupsel de Azevedo, Bill Doyle, Christopher A. Fiebrich, and David Schvartzman
Atmos. Meas. Tech., 15, 5599–5618, https://doi.org/10.5194/amt-15-5599-2022, https://doi.org/10.5194/amt-15-5599-2022, 2022
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Strong changes in pressure, temperature, and humidity occur when small scientific aircraft ascend through the atmosphere to measure carbon dioxide. These strong changes can produce errors in the carbon dioxide measurements. To avoid these errors, we present a low-cost and simple correction method. This low-complexity method allows more researchers to study atmospheric carbon dioxide, reducing entry barriers in this field.
Ilann Bourgeois, Jeff Peischl, J. Andrew Neuman, Steven S. Brown, Hannah M. Allen, Pedro Campuzano-Jost, Matthew M. Coggon, Joshua P. DiGangi, Glenn S. Diskin, Jessica B. Gilman, Georgios I. Gkatzelis, Hongyu Guo, Hannah A. Halliday, Thomas F. Hanisco, Christopher D. Holmes, L. Gregory Huey, Jose L. Jimenez, Aaron D. Lamplugh, Young Ro Lee, Jakob Lindaas, Richard H. Moore, Benjamin A. Nault, John B. Nowak, Demetrios Pagonis, Pamela S. Rickly, Michael A. Robinson, Andrew W. Rollins, Vanessa Selimovic, Jason M. St. Clair, David Tanner, Krystal T. Vasquez, Patrick R. Veres, Carsten Warneke, Paul O. Wennberg, Rebecca A. Washenfelder, Elizabeth B. Wiggins, Caroline C. Womack, Lu Xu, Kyle J. Zarzana, and Thomas B. Ryerson
Atmos. Meas. Tech., 15, 4901–4930, https://doi.org/10.5194/amt-15-4901-2022, https://doi.org/10.5194/amt-15-4901-2022, 2022
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Understanding fire emission impacts on the atmosphere is key to effective air quality management and requires accurate measurements. We present a comparison of airborne measurements of key atmospheric species in ambient air and in fire smoke. We show that most instruments performed within instrument uncertainties. In some cases, further work is needed to fully characterize instrument performance. Comparing independent measurements using different techniques is important to assess their accuracy.
Woohui Nam, Changmin Cho, Begie Perdigones, Tae Siek Rhee, and Kyung-Eun Min
Atmos. Meas. Tech., 15, 4473–4487, https://doi.org/10.5194/amt-15-4473-2022, https://doi.org/10.5194/amt-15-4473-2022, 2022
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We describe our vibration-resistant instrument for measuring ambient NO3, NO2, and H2O based on cavity-enhanced absorption spectroscopy. By simultaneous retrieval of H2O with the other species using a measured H2O absorption spectrum, direct quantifications among all species are possible without any pre-treatment for H2O. Our instrument achieves the effective light path to ~101.5 km, which allows the sensitive measurements of NO3 and NO2 as 1.41 pptv and 6.92 ppbv (1σ) in 1 s.
Yunsong Liu, Jean-Daniel Paris, Mihalis Vrekoussis, Panayiota Antoniou, Christos Constantinides, Maximilien Desservettaz, Christos Keleshis, Olivier Laurent, Andreas Leonidou, Carole Philippon, Panagiotis Vouterakos, Pierre-Yves Quéhé, Philippe Bousquet, and Jean Sciare
Atmos. Meas. Tech., 15, 4431–4442, https://doi.org/10.5194/amt-15-4431-2022, https://doi.org/10.5194/amt-15-4431-2022, 2022
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This paper details laboratory-based and field developments of a cost-effective and compacted UAV CO2 sensor system to address the challenge of measuring CO2 with sufficient precision and acquisition frequency. We assess its performance extensively through laboratory and field tests and provide a case study in an urban area (Nicosia, Cyprus). We therefore expect that this portable system will be widely used for measuring CO2 emission and distribution in natural or urban environments.
Subin Yoon, Alexander Kotsakis, Sergio L. Alvarez, Mark G. Spychala, Elizabeth Klovenski, Paul Walter, Gary Morris, Ernesto Corrales, Alfredo Alan, Jorge A. Diaz, and James H. Flynn
Atmos. Meas. Tech., 15, 4373–4384, https://doi.org/10.5194/amt-15-4373-2022, https://doi.org/10.5194/amt-15-4373-2022, 2022
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SO2 is adverse to human health and the environment. A single SO2 sonde was developed to provide direct SO2 measurement with a greater vertical extent, a lower limit of detection, and less uncertainty relative to the previous dual-sonde method. The single sonde was tested in the field near volcanoes and anthropogenic sources where the sonde measured SO2 ranging from 0.5 to 940 ppb. This lighter-weight payload can be a great candidate to attach to small drones and unmanned aerial vehicles.
Michael A. Robinson, J. Andrew Neuman, L. Gregory Huey, James M. Roberts, Steven S. Brown, and Patrick R. Veres
Atmos. Meas. Tech., 15, 4295–4305, https://doi.org/10.5194/amt-15-4295-2022, https://doi.org/10.5194/amt-15-4295-2022, 2022
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Iodide chemical ionization mass spectrometry (CIMS) is commonly used in atmospheric chemistry laboratory studies and field campaigns. Deployment of the NOAA iodide CIMS instrument in the summer of 2021 indicated a significant and overlooked temperature dependence of the instrument sensitivity. This work explores which analytes are influenced by this phenomena. Additionally, we recommend controls to reduce this effect for future field deployments.
Roland Vernooij, Patrik Winiger, Martin Wooster, Tercia Strydom, Laurent Poulain, Ulrike Dusek, Mark Grosvenor, Gareth J. Roberts, Nick Schutgens, and Guido R. van der Werf
Atmos. Meas. Tech., 15, 4271–4294, https://doi.org/10.5194/amt-15-4271-2022, https://doi.org/10.5194/amt-15-4271-2022, 2022
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Landscape fires are a substantial emitter of greenhouse gases and aerosols. Previous studies have indicated savanna emission factors to be highly variable. Improving fire emission estimates, and understanding future climate- and human-induced changes in fire regimes, requires in situ measurements. We present a drone-based method that enables the collection of a large amount of high-quality emission factor measurements that do not have the biases of aircraft or surface measurements.
Ralf Tillmann, Georgios I. Gkatzelis, Franz Rohrer, Benjamin Winter, Christian Wesolek, Tobias Schuldt, Anne C. Lange, Philipp Franke, Elmar Friese, Michael Decker, Robert Wegener, Morten Hundt, Oleg Aseev, and Astrid Kiendler-Scharr
Atmos. Meas. Tech., 15, 3827–3842, https://doi.org/10.5194/amt-15-3827-2022, https://doi.org/10.5194/amt-15-3827-2022, 2022
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We report in situ measurements of air pollutant concentrations within the planetary boundary layer on board a Zeppelin in Germany. The low costs of commercial flights provide an affordable and efficient method to improve our understanding of changes in emissions in space and time. The experimental setup expands the capabilities of this platform and provides insights into primary and secondary pollution observations and planetary boundary layer dynamics which determine air quality significantly.
Mei Bai, Zoe Loh, David W. T. Griffith, Debra Turner, Richard Eckard, Robert Edis, Owen T. Denmead, Glenn W. Bryant, Clare Paton-Walsh, Matthew Tonini, Sean M. McGinn, and Deli Chen
Atmos. Meas. Tech., 15, 3593–3610, https://doi.org/10.5194/amt-15-3593-2022, https://doi.org/10.5194/amt-15-3593-2022, 2022
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The open-path laser (OPL) and open-path Fourier transform infrared (OP-FTIR) are used in agricultural research, but their error in emissions research has not been the focus of studies. We conducted trace gas release trials and herd and paddock emission studies to compare their applicability and performance. The OP-FTIR has better stability in stable conditions than OPL. The CH4 OPL accurately detects the low background level of CH4, but the NH3 OPL only detects background values >10 ppbv.
Roger Curcoll, Josep-Anton Morguí, Armand Kamnang, Lídia Cañas, Arturo Vargas, and Claudia Grossi
Atmos. Meas. Tech., 15, 2807–2818, https://doi.org/10.5194/amt-15-2807-2022, https://doi.org/10.5194/amt-15-2807-2022, 2022
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Low-cost air enquirer kits, including CO2 and environmental parameter sensors, have been designed, built, and tested in a new steady-state through-flow chamber for simultaneous measurements of CO2 fluxes in soil and CO2 concentrations in air. A CO2 calibration and multiparametric fitting reduced the total uncertainty of CO2 concentration by 90 %. This system allows continuous measurement of CO2 fluxes and CO2 ambient air, with low cost (EUR 1200), low energy demand (<5 W), and low maintenance.
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Short summary
This paper describes the measurement of atomic oxygen in the upper atmosphere onboard sounding rockets using solid electrolyte sensors. Calibration of the sensors in the laboratory is explained in detail. Results from the WADIS-2 rocket campaign show profiles of atomic oxygen density with a high spatial resolution.
This paper describes the measurement of atomic oxygen in the upper atmosphere onboard sounding...
