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Atmospheric Measurement Techniques An interactive open-access journal of the European Geosciences Union

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Atmos. Meas. Tech., 5, 1627-1635, 2012
https://doi.org/10.5194/amt-5-1627-2012
© Author(s) 2012. This work is distributed under
the Creative Commons Attribution 3.0 License.
Research article
12 Jul 2012
Remote sensing of CO2 and CH4 using solar absorption spectrometry with a low resolution spectrometer
C. Petri1, T. Warneke1, N. Jones2, T. Ridder1, J. Messerschmidt1, T. Weinzierl1, M. Geibel3,*, and J. Notholt1 1IUP, University of Bremen, Bremen, Germany
2School of Chemistry, University of Wollongong, Wollongong, Australia
3Max Planck Institute for Biogeochemistry, Jena, Germany
*now at: Department for Applied Environmental Research (ITM), Stockholm University, Stockholm, Sweden
Abstract. Throughout the last few years solar absorption Fourier Transform Spectrometry (FTS) has been further developed to measure the total columns of CO2 and CH4. The observations are performed at high spectral resolution, typically at 0.02 cm−1. The precision currently achieved is generally better than 0.25%. However, these high resolution instruments are quite large and need a dedicated room or container for installation. We performed these observations using a smaller commercial interferometer at its maximum possible resolution of 0.11 cm−1. The measurements have been performed at Bremen and have been compared to observations using our high resolution instrument also situated at the same location. The high resolution instrument has been successfully operated as part of the Total Carbon Column Observing Network (TCCON). The precision of the low resolution instrument is 0.32% for XCO2 and 0.46% for XCH4. A comparison of the measurements of both instruments yields an average deviation in the retrieved daily means of ≤0.2% for CO2. For CH4 an average bias between the instruments of 0.47% was observed. For test cases, spectra recorded by the high resolution instrument have been truncated to the resolution of 0.11 cm−1. This study gives an offset of 0.03% for CO2 and 0.26% for CH4. These results indicate that for CH4 more than 50% of the difference between the instruments results from the resolution dependent retrieval. We tentatively assign the offset to an incorrect a-priori concentration profile or the effect of interfering gases, which may not be treated correctly.

Citation: Petri, C., Warneke, T., Jones, N., Ridder, T., Messerschmidt, J., Weinzierl, T., Geibel, M., and Notholt, J.: Remote sensing of CO2 and CH4 using solar absorption spectrometry with a low resolution spectrometer, Atmos. Meas. Tech., 5, 1627-1635, https://doi.org/10.5194/amt-5-1627-2012, 2012.
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