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Atmospheric Measurement Techniques An interactive open-access journal of the European Geosciences Union
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Volume 5, issue 8 | Copyright
Atmos. Meas. Tech., 5, 2057-2068, 2012
https://doi.org/10.5194/amt-5-2057-2012
© Author(s) 2012. This work is distributed under
the Creative Commons Attribution 3.0 License.

Research article 24 Aug 2012

Research article | 24 Aug 2012

DOAS measurements of NO2 from an ultralight aircraft during the Earth Challenge expedition

A. Merlaud1, M. Van Roozendael1, J. van Gent1, C. Fayt1, J. Maes1, X. Toledo-Fuentes2, O. Ronveaux3, and M. De Mazière1 A. Merlaud et al.
  • 1Belgian Insitute for Space Aeronomy (BIRA-IASB), Avenue Circulaire 3, 1180 Brussels, Belgium
  • 2Research Centre in Physics of Matter and Radiation (PMR), University of Namur, Rue de Bruxelles 61, 5000 Namur, Belgium
  • 3Usf-free sky, Rue du Page 65, 1050 Brussels, Belgium

Abstract. We report on airborne Differential Optical Absorption Spectroscopy (DOAS) measurements of NO2 tropospheric columns above South Asia, the Arabic peninsula, North Africa, and Italy in November and December 2009. The DOAS instrument was installed on an ultralight aircraft involved in the Earth Challenge project, an expedition of seven pilots flying on four ultralight aircraft between Australia and Belgium. The instrument recorded spectra in limb geometry with a large field of view, a set-up which provides a high sensitivity to the boundary layer NO2 while minimizing the uncertainties related to the attitude variations. We compare our measurements with OMI (Ozone Monitoring Instrument) and GOME-2 (Global Ozone Monitoring Experiment 2) tropospheric NO2 products when the latter are available. Above Rajasthan and the Po Valley, two areas where the NO2 field is homogeneous, data sets agree very well. Our measurements in these areas are 0.1 ± 0.1 to 3 ± 1 × 1015 molec cm−2 and 2.6 ± 0.8 × 1016 molec cm−2, respectively. Flying downwind of Riyadh, our NO2 measurements show the structure of the megacity's exhaust plume with a higher spatial resolution than OMI. Moreover, our measurements are larger (up to 40%) than those seen by satellites. We also derived tropospheric columns when no satellite data were available if it was possible to get information on the visibility from satellite measurements of aerosol optical thickness. This experiment also provides a confirmation for the recent finding of a soil signature above desert.

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