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Atmospheric Measurement Techniques An interactive open-access journal of the European Geosciences Union
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Volume 5, issue 11
Atmos. Meas. Tech., 5, 2601–2611, 2012
https://doi.org/10.5194/amt-5-2601-2012
© Author(s) 2012. This work is distributed under
the Creative Commons Attribution 3.0 License.
Atmos. Meas. Tech., 5, 2601–2611, 2012
https://doi.org/10.5194/amt-5-2601-2012
© Author(s) 2012. This work is distributed under
the Creative Commons Attribution 3.0 License.

Research article 01 Nov 2012

Research article | 01 Nov 2012

Ground-based millimeter-wave observation of stratospheric ClO over Atacama, Chile in the mid-latitude Southern Hemisphere

T. Kuwahara1, T. Nagahama1, H. Maezawa2, Y. Kojima1, H. Yamamoto3, T. Okuda3, N. Mizuno4, H. Nakane5, Y. Fukui3, and A. Mizuno1 T. Kuwahara et al.
  • 1Solar-Terrestrial Environment Laboratory, Nagoya University, Nagoya, Aichi, Japan
  • 2Department of Physics, Osaka Prefecture University, Sakai, Osaka, Japan
  • 3Department of Astrophysics, Nagoya University, Nagoya, Aichi, Japan
  • 4National Astronomical Observatory of Japan, Mitaka, Tokyo, Japan
  • 5National Institute for Environmental Studies, Tsukuba, Ibaraki, Japan

Abstract. We have performed ground-based measurements of stratospheric chlorine monoxide (ClO) during the summer in 2009 over the Atacama highland, Chile, a new observing site in the mid-latitude region in the Southern Hemisphere, by using a millimeter-wave spectroscopic radiometer. The radiometer, equipped with a superconducting receiver and a digital Fourier spectrometer, was developed by Nagoya University, and the new observing system provides us high sensitivity and stable performance to measure the very weak ClO lines. The receiver noise temperature of the superconducting receiver is 170 K in DSB. To reveal the diurnal variation of ClO, we retrieved the vertical mixing ratio profiles by the weighted-damped least-squares algorithm applied for the spectral data at 203 GHz obtained between 5 and 16 December 2009. The total error on the retrieval is estimated to be 20% to 30% in an altitude range from 40 km to 50 km. The amplitude of the diurnal variation is estimated as 33% of the daytime average at 40 km. The observed time variation shows a pattern similar to that of the previous works observed in the northern mid-latitude region.

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