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Atmospheric Measurement Techniques An interactive open-access journal of the European Geosciences Union

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Atmos. Meas. Tech., 6, 63-79, 2013
https://doi.org/10.5194/amt-6-63-2013
© Author(s) 2013. This work is distributed under
the Creative Commons Attribution 3.0 License.
Research article
10 Jan 2013
Profiling tropospheric CO2 using Aura TES and TCCON instruments
L. Kuai1, J. Worden1, S. Kulawik1, K. Bowman1, M. Lee1, S. C. Biraud2, J. B. Abshire3, S. C. Wofsy4, V. Natraj1, C. Frankenberg1, D. Wunch5, B. Connor6, C. Miller1, C. Roehl5, R.-L. Shia5, and Y. Yung5 1Jet Propulsion Laboratory, California Institute of Technology, 4800 Oak Grove Drive, Mail stop: 233-200, Pasadena, CA 91109, USA
2Lawrence Berkeley National Laboratories, Berkeley, CA 94720, USA
3NASA Goddard Space Flight Center, Greenbelt, MD, USA
4Harvard University, Cambridge, MA, USA
5California Institute of Technology, 1200 E. California Blvd., Pasadena, CA 91125, USA
6BC Consulting Ltd., 6 Fairway Dr., Alexandra, 9320, New Zealand
Abstract. Monitoring the global distribution and long-term variations of CO2 sources and sinks is required for characterizing the global carbon budget. Total column measurements are useful for estimating regional-scale fluxes; however, model transport remains a significant error source, particularly for quantifying local sources and sinks. To improve the capability of estimating regional fluxes, we estimate lower tropospheric CO2 concentrations from ground-based near-infrared (NIR) measurements with space-based thermal infrared (TIR) measurements. The NIR measurements are obtained from the Total Carbon Column Observing Network (TCCON) of solar measurements, which provide an estimate of the total CO2 column amount. Estimates of tropospheric CO2 that are co-located with TCCON are obtained by assimilating Tropospheric Emission Spectrometer (TES) free tropospheric CO2 estimates into the GEOS-Chem model. We find that quantifying lower tropospheric CO2 by subtracting free tropospheric CO2 estimates from total column estimates is a linear problem, because the calculated random uncertainties in total column and lower tropospheric estimates are consistent with actual uncertainties as compared to aircraft data. For the total column estimates, the random uncertainty is about 0.55 ppm with a bias of −5.66 ppm, consistent with previously published results. After accounting for the total column bias, the bias in the lower tropospheric CO2 estimates is 0.26 ppm with a precision (one standard deviation) of 1.02 ppm. This precision is sufficient for capturing the winter to summer variability of approximately 12 ppm in the lower troposphere; double the variability of the total column. This work shows that a combination of NIR and TIR measurements can profile CO2 with the precision and accuracy needed to quantify lower tropospheric CO2 variability.

Citation: Kuai, L., Worden, J., Kulawik, S., Bowman, K., Lee, M., Biraud, S. C., Abshire, J. B., Wofsy, S. C., Natraj, V., Frankenberg, C., Wunch, D., Connor, B., Miller, C., Roehl, C., Shia, R.-L., and Yung, Y.: Profiling tropospheric CO2 using Aura TES and TCCON instruments, Atmos. Meas. Tech., 6, 63-79, https://doi.org/10.5194/amt-6-63-2013, 2013.
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