Articles | Volume 8, issue 8
https://doi.org/10.5194/amt-8-3337-2015
© Author(s) 2015. This work is distributed under
the Creative Commons Attribution 3.0 License.
the Creative Commons Attribution 3.0 License.
https://doi.org/10.5194/amt-8-3337-2015
© Author(s) 2015. This work is distributed under
the Creative Commons Attribution 3.0 License.
the Creative Commons Attribution 3.0 License.
Research article
| 
18 Aug 2015
Research article |
| 18 Aug 2015
Hyphenation of a EC / OC thermal–optical carbon analyzer to photo-ionization time-of-flight mass spectrometry: an off-line aerosol mass spectrometric approach for characterization of primary and secondary particulate matter
J. Diab
Joint Mass Spectrometry Centre/Chair of Analytical Chemistry, University of Rostock, 18051 Rostock, Germany
T. Streibel
Joint Mass Spectrometry Centre/Chair of Analytical Chemistry, University of Rostock, 18051 Rostock, Germany
Joint Mass Spectrometry Centre/Institute of Ecological Chemistry, Helmholtz Centre Munich, Research Centre for Environmental Health (GmbH), 85764 Munich, Germany
F. Cavalli
JRC European Commission – Joint Research Centre, Institute for Environment and Sustainability – Air & Climate Unit, 21027 Ispra, Italy
S. C. Lee
The Hong Kong Polytechnic University, Department of Civil & Structural Engineering, Hung Hom, Kowloon, Hong Kong, China
H. Saathoff
Karlsruhe Institute of Technology (KIT), Institute for Meteorology and Climate Research, Atmospheric Aerosol Research Division, 76344 Eggenstein-Leopoldshafen, Germany
A. Mamakos
JRC European Commission – Joint Research Centre, Institute for Energy – Sustainable Transport Unit, 21027 Ispra, Italy
J. C. Chow
DRI-Desert Research Institute, Division of Atmospheric sciences, Reno, NV 89512, USA
L.-W. A. Chen
Department of Environmental and Occupational Health, University of Nevada, Las Vegas, NV 89154, USA
J. G. Watson
DRI-Desert Research Institute, Division of Atmospheric sciences, Reno, NV 89512, USA
O. Sippula
Joint Mass Spectrometry Centre/Chair of Analytical Chemistry, University of Rostock, 18051 Rostock, Germany
Department of Environmental Science, University of Eastern Finland, P.O. Box 1627, 70211, Kuopio, Finland
R. Zimmermann
CORRESPONDING AUTHOR
Joint Mass Spectrometry Centre/Chair of Analytical Chemistry, University of Rostock, 18051 Rostock, Germany
Joint Mass Spectrometry Centre/Institute of Ecological Chemistry, Helmholtz Centre Munich, Research Centre for Environmental Health (GmbH), 85764 Munich, Germany
Viewed
Total article views: 3,888 (including HTML, PDF, and XML)
Cumulative views and downloads
(calculated since 08 Jan 2015)
| HTML | XML | Total | Supplement | BibTeX | EndNote | |
|---|---|---|---|---|---|---|
| 2,123 | 1,438 | 327 | 3,888 | 821 | 114 | 133 |
- HTML: 2,123
- PDF: 1,438
- XML: 327
- Total: 3,888
- Supplement: 821
- BibTeX: 114
- EndNote: 133
Total article views: 2,825 (including HTML, PDF, and XML)
Cumulative views and downloads
(calculated since 18 Aug 2015)
| HTML | XML | Total | Supplement | BibTeX | EndNote | |
|---|---|---|---|---|---|---|
| 1,640 | 1,044 | 141 | 2,825 | 635 | 81 | 105 |
- HTML: 1,640
- PDF: 1,044
- XML: 141
- Total: 2,825
- Supplement: 635
- BibTeX: 81
- EndNote: 105
Total article views: 1,063 (including HTML, PDF, and XML)
Cumulative views and downloads
(calculated since 08 Jan 2015)
| HTML | XML | Total | BibTeX | EndNote | |
|---|---|---|---|---|---|
| 483 | 394 | 186 | 1,063 | 33 | 28 |
- HTML: 483
- PDF: 394
- XML: 186
- Total: 1,063
- BibTeX: 33
- EndNote: 28
Cited
29 citations as recorded by crossref.
- Review on recent progress in observations, source identifications and countermeasures of PM2.5 C. Liang et al. 10.1016/j.envint.2015.10.016
- Review on Evolved Gas Analysis Mass Spectrometry with Soft Photoionization for the Chemical Description of Petroleum, Petroleum-Derived Materials, and Alternative Feedstocks C. Rüger et al. 10.1021/acs.energyfuels.1c02720
- A chemometric investigation of aromatic emission profiles from a marine engine in comparison with residential wood combustion and road traffic: Implications for source apportionment inside and outside sulphur emission control areas H. Czech et al. 10.1016/j.atmosenv.2017.08.022
- Mass spectrometric analysis of unprecedented high levels of carbonaceous aerosol particles long-range transported from wildfires in the Siberian Arctic E. Schneider et al. 10.5194/acp-24-553-2024
- Atomic spectrometry update – a review of advances in environmental analysis O. Butler et al. 10.1039/C5JA90061A
- Brown Coal and Logwood Combustion in a Modern Heating Appliance: The Impact of Combustion Quality and Fuel on Organic Aerosol Composition P. Martens et al. 10.1021/acs.est.2c08787
- Toxicity of Water- and Organic-Soluble Wood Tar Fractions from Biomass Burning in Lung Epithelial Cells M. Pardo et al. 10.1021/acs.chemrestox.1c00020
- Quantification of long-term primary and secondary source contributions to carbonaceous aerosols G. Shi et al. 10.1016/j.envpol.2016.09.009
- Impact of Thermal Stress on Abrasive Dust from a Carbon Fiber-Reinforced Concrete Composite A. Koch et al. 10.3390/fib10050039
- Development and Application of Photoionization Technology for Organic Analysis of Particulate Matter M. Yuan & J. Cao 10.1007/s41810-022-00130-z
- Vacuum Laser Photoionization inside the C-trap of an Orbitrap Mass Spectrometer: Resonance-Enhanced Multiphoton Ionization High-Resolution Mass Spectrometry P. Kösling et al. 10.1021/acs.analchem.1c01018
- Chemical composition and speciation of particulate organic matter from modern residential small-scale wood combustion appliances H. Czech et al. 10.1016/j.scitotenv.2017.08.263
- Composition of carbonaceous fine particulate emissions of a flexible fuel DISI engine under high velocity and municipal conditions T. Miersch et al. 10.1016/j.fuel.2018.09.136
- Emission characteristics and optical properties of brown carbon during combustion of pine at different ignition temperatures under high-time resolution J. Cai et al. 10.1016/j.fuel.2023.129400
- Addressing Thermal Behavior and Molecular Architecture of Asphaltenes by a Thermal-Optical Carbon Analyzer Coupled to High-Resolution Mass Spectrometry C. Rüger et al. 10.1021/acs.energyfuels.2c02122
- Secondary organic aerosols produced from photochemical oxidation of secondarily evaporated biomass burning organic gases: Chemical composition, toxicity, optical properties, and climate effect Z. Fang et al. 10.1016/j.envint.2021.106801
- Impact of photochemical ageing on Polycyclic Aromatic Hydrocarbons (PAH) and oxygenated PAH (Oxy-PAH/OH-PAH) in logwood stove emissions T. Miersch et al. 10.1016/j.scitotenv.2019.05.412
- Umweltanalytik: Smoke on the Water: Rußpartikel aus Schiffen H. Czech et al. 10.1002/nadc.20184080756
- Investigation of Chemical Composition and Fiber-Occurrence in Inhalable Particulate Matter Obtained from Dry Cutting Processes of Carbon Fiber Reinforced Concrete Composite, Concrete and the Carbon Fiber Reinforcement Materials A. Koch et al. 10.1007/s41810-021-00103-8
- Traceability tagging of volatile organic compound sources and their contributions to ozone formation in Suzhou using vehicle-based portable single-photon ionization mass spectrometry N. Shuaibu et al. 10.1186/s12302-024-00872-2
- Aerosol emissions of a ship diesel engine operated with diesel fuel or heavy fuel oil T. Streibel et al. 10.1007/s11356-016-6724-z
- Feasibility of coupling a thermal/optical carbon analyzer to a quadrupole mass spectrometer for enhanced PM2.5 speciation G. Riggio et al. 10.1080/10962247.2017.1394928
- Impacts of peat-forest smoke on urban PM2.5 in the Maritime Continent during 2012–2015: Carbonaceous profiles and indicators J. Tham et al. 10.1016/j.envpol.2019.02.049
- Air quality measurements—From rubber bands to tapping the rainbow G. Hidy et al. 10.1080/10962247.2017.1308890
- Summertime Day-Night Differences of PM2.5 Components (Inorganic Ions, OC, EC, WSOC, WSON, HULIS, and PAHs) in Changzhou, China Z. Ye et al. 10.3390/atmos8100189
- A study on the chemical profile and the derived health effects of heavy-duty machinery aerosol with a focus on the impact of alternative fuels N. Gawlitta et al. 10.1007/s11869-022-01287-9
- A novel measurement system for unattended, in situ characterization of carbonaceous aerosols A. Keller et al. 10.5194/ar-1-65-2023
- PM2.5 source apportionment with organic markers in the Southeastern Aerosol Research and Characterization (SEARCH) study J. Watson et al. 10.1080/10962247.2015.1063551
- A comparative study on the size distribution and carbon components of particulate matters from typical sources L. Zuo et al. 10.1002/ep.13462
27 citations as recorded by crossref.
- Review on recent progress in observations, source identifications and countermeasures of PM2.5 C. Liang et al. 10.1016/j.envint.2015.10.016
- Review on Evolved Gas Analysis Mass Spectrometry with Soft Photoionization for the Chemical Description of Petroleum, Petroleum-Derived Materials, and Alternative Feedstocks C. Rüger et al. 10.1021/acs.energyfuels.1c02720
- A chemometric investigation of aromatic emission profiles from a marine engine in comparison with residential wood combustion and road traffic: Implications for source apportionment inside and outside sulphur emission control areas H. Czech et al. 10.1016/j.atmosenv.2017.08.022
- Mass spectrometric analysis of unprecedented high levels of carbonaceous aerosol particles long-range transported from wildfires in the Siberian Arctic E. Schneider et al. 10.5194/acp-24-553-2024
- Atomic spectrometry update – a review of advances in environmental analysis O. Butler et al. 10.1039/C5JA90061A
- Brown Coal and Logwood Combustion in a Modern Heating Appliance: The Impact of Combustion Quality and Fuel on Organic Aerosol Composition P. Martens et al. 10.1021/acs.est.2c08787
- Toxicity of Water- and Organic-Soluble Wood Tar Fractions from Biomass Burning in Lung Epithelial Cells M. Pardo et al. 10.1021/acs.chemrestox.1c00020
- Quantification of long-term primary and secondary source contributions to carbonaceous aerosols G. Shi et al. 10.1016/j.envpol.2016.09.009
- Impact of Thermal Stress on Abrasive Dust from a Carbon Fiber-Reinforced Concrete Composite A. Koch et al. 10.3390/fib10050039
- Development and Application of Photoionization Technology for Organic Analysis of Particulate Matter M. Yuan & J. Cao 10.1007/s41810-022-00130-z
- Vacuum Laser Photoionization inside the C-trap of an Orbitrap Mass Spectrometer: Resonance-Enhanced Multiphoton Ionization High-Resolution Mass Spectrometry P. Kösling et al. 10.1021/acs.analchem.1c01018
- Chemical composition and speciation of particulate organic matter from modern residential small-scale wood combustion appliances H. Czech et al. 10.1016/j.scitotenv.2017.08.263
- Composition of carbonaceous fine particulate emissions of a flexible fuel DISI engine under high velocity and municipal conditions T. Miersch et al. 10.1016/j.fuel.2018.09.136
- Emission characteristics and optical properties of brown carbon during combustion of pine at different ignition temperatures under high-time resolution J. Cai et al. 10.1016/j.fuel.2023.129400
- Addressing Thermal Behavior and Molecular Architecture of Asphaltenes by a Thermal-Optical Carbon Analyzer Coupled to High-Resolution Mass Spectrometry C. Rüger et al. 10.1021/acs.energyfuels.2c02122
- Secondary organic aerosols produced from photochemical oxidation of secondarily evaporated biomass burning organic gases: Chemical composition, toxicity, optical properties, and climate effect Z. Fang et al. 10.1016/j.envint.2021.106801
- Impact of photochemical ageing on Polycyclic Aromatic Hydrocarbons (PAH) and oxygenated PAH (Oxy-PAH/OH-PAH) in logwood stove emissions T. Miersch et al. 10.1016/j.scitotenv.2019.05.412
- Umweltanalytik: Smoke on the Water: Rußpartikel aus Schiffen H. Czech et al. 10.1002/nadc.20184080756
- Investigation of Chemical Composition and Fiber-Occurrence in Inhalable Particulate Matter Obtained from Dry Cutting Processes of Carbon Fiber Reinforced Concrete Composite, Concrete and the Carbon Fiber Reinforcement Materials A. Koch et al. 10.1007/s41810-021-00103-8
- Traceability tagging of volatile organic compound sources and their contributions to ozone formation in Suzhou using vehicle-based portable single-photon ionization mass spectrometry N. Shuaibu et al. 10.1186/s12302-024-00872-2
- Aerosol emissions of a ship diesel engine operated with diesel fuel or heavy fuel oil T. Streibel et al. 10.1007/s11356-016-6724-z
- Feasibility of coupling a thermal/optical carbon analyzer to a quadrupole mass spectrometer for enhanced PM2.5 speciation G. Riggio et al. 10.1080/10962247.2017.1394928
- Impacts of peat-forest smoke on urban PM2.5 in the Maritime Continent during 2012–2015: Carbonaceous profiles and indicators J. Tham et al. 10.1016/j.envpol.2019.02.049
- Air quality measurements—From rubber bands to tapping the rainbow G. Hidy et al. 10.1080/10962247.2017.1308890
- Summertime Day-Night Differences of PM2.5 Components (Inorganic Ions, OC, EC, WSOC, WSON, HULIS, and PAHs) in Changzhou, China Z. Ye et al. 10.3390/atmos8100189
- A study on the chemical profile and the derived health effects of heavy-duty machinery aerosol with a focus on the impact of alternative fuels N. Gawlitta et al. 10.1007/s11869-022-01287-9
- A novel measurement system for unattended, in situ characterization of carbonaceous aerosols A. Keller et al. 10.5194/ar-1-65-2023
2 citations as recorded by crossref.
- PM2.5 source apportionment with organic markers in the Southeastern Aerosol Research and Characterization (SEARCH) study J. Watson et al. 10.1080/10962247.2015.1063551
- A comparative study on the size distribution and carbon components of particulate matters from typical sources L. Zuo et al. 10.1002/ep.13462
Saved (final revised paper)
Saved (final revised paper)
Saved (preprint)
Latest update: 23 Apr 2024
Short summary
This paper depicts several fields of application of a new analytical method, which expands the well-established EC/OC method, which enables one to measure the carbon content (organic and elemental) of particulate aerosols. It was coupled to photo-ionization mass spectrometry to get structural information of the evolving carbonaceous species. Application fields such as smoke chamber-, ambient - and wood combustion particles were addressed, covering exemplary primary and secondary aerosol sources.
This paper depicts several fields of application of a new analytical method, which expands the...
