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Volume 8, issue 8
Atmos. Meas. Tech., 8, 3537–3553, 2015
https://doi.org/10.5194/amt-8-3537-2015
© Author(s) 2015. This work is distributed under
the Creative Commons Attribution 3.0 License.
Atmos. Meas. Tech., 8, 3537–3553, 2015
https://doi.org/10.5194/amt-8-3537-2015
© Author(s) 2015. This work is distributed under
the Creative Commons Attribution 3.0 License.

Research article 31 Aug 2015

Research article | 31 Aug 2015

Detailed characterizations of the new Mines Douai comparative reactivity method instrument via laboratory experiments and modeling

V. Michoud et al.
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Cited articles  
Atkinson, R., Aschmann, S. M., Winer, A. M. and Carter, W. P. L.: Rate constants for the gas phase reactions of OH radicals and O3 with pyrrole at 295 ± 1 K and atmospheric pressure, Atmos. Environ. 1967, 18, 2105–2107, https://doi.org/10.1016/0004-6981(84)90196-3, 1984.
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Calpini, B., Jeanneret, F., Bourqui, M., Clappier, A., Vajtai, R. and van den Bergh, H.: Direct measurement of the total reaction rate of OH in the atmosphere, Analusis, 27, 328–336, https://doi.org/10.1051/analusis:1999270328, 1999.
Carslaw, N., Creasey, D. J., Heard, D. E., Jacobs, P. J., Lee, J. D., Lewis, A. C., McQuaid, J. B., Pilling, M. J., Bauguitte, S., Penkett, S. A., Monks, P. S., and Salisbury, G.: Eastern Atlantic Spring Experiment 1997 (EASE97) – 2. Comparisons of model concentrations of OH, HO2, and RO2 with measurements, J. Geophys. Res., 107, 4190, https://doi.org/10.1029/2001JD001568, 2002.
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This study presents the results of an exhaustive characterization of a CRM instrument developed at Mines Douai to measure total OH reactivity in the troposphere. To do so, a suite of laboratory experiments was conducted to assess the different corrections that need to be applied during data processing. The results were then compared to simulations from a 0-D box model, including two different chemical mechanisms, leading to reasonable agreement.
This study presents the results of an exhaustive characterization of a CRM instrument developed...
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