Articles | Volume 8, issue 11
https://doi.org/10.5194/amt-8-4803-2015
© Author(s) 2015. This work is distributed under
the Creative Commons Attribution 3.0 License.
the Creative Commons Attribution 3.0 License.
https://doi.org/10.5194/amt-8-4803-2015
© Author(s) 2015. This work is distributed under
the Creative Commons Attribution 3.0 License.
the Creative Commons Attribution 3.0 License.
Research article
| 
18 Nov 2015
Research article |
| 18 Nov 2015
Characterization of trace metals on soot aerosol particles with the SP-AMS: detection and quantification
S. Carbone
CORRESPONDING AUTHOR
Atmospheric Composition Research, Finnish Meteorological Institute, P.O. Box 503, 00101 Helsinki, Finland
now at: Department of Applied Physics, University of São Paulo, São Paulo, Brazil
T. Onasch
Aerodyne Research, Inc. 45 Manning Road, 01821-3976, Billerica, MA, USA
S. Saarikoski
Atmospheric Composition Research, Finnish Meteorological Institute, P.O. Box 503, 00101 Helsinki, Finland
H. Timonen
Atmospheric Composition Research, Finnish Meteorological Institute, P.O. Box 503, 00101 Helsinki, Finland
K. Saarnio
Atmospheric Composition Research, Finnish Meteorological Institute, P.O. Box 503, 00101 Helsinki, Finland
D. Sueper
Aerodyne Research, Inc. 45 Manning Road, 01821-3976, Billerica, MA, USA
Cooperative Institute for Research In Environmental Sciences, University of Colorado, Boulder, CO 80303, USA
T. Rönkkö
Tampere University of Technology, Department of Physics, Tampere, Finland
L. Pirjola
Department of Physics, University of Helsinki, P.O. Box 64, 00014 Helsinki, Finland
Metropolia University of Applied Sciences, P.O. Box 4021, Helsinki, Finland
A. Häyrinen
Helen Ltd., 00090 Helen, Helsinki, Finland
D. Worsnop
Atmospheric Composition Research, Finnish Meteorological Institute, P.O. Box 503, 00101 Helsinki, Finland
Aerodyne Research, Inc. 45 Manning Road, 01821-3976, Billerica, MA, USA
Department of Physics, University of Helsinki, P.O. Box 64, 00014 Helsinki, Finland
R. Hillamo
Atmospheric Composition Research, Finnish Meteorological Institute, P.O. Box 503, 00101 Helsinki, Finland
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Cited
26 citations as recorded by crossref.
- Influence of Emissions and Aqueous Processing on Particles Containing Black Carbon in a Polluted Urban Environment: Insights From a Soot Particle‐Aerosol Mass Spectrometer S. Collier et al. 10.1002/2017JD027851
- Technical note: A new approach to discriminate different black carbon sources by utilising fullerene and metals in positive matrix factorisation analysis of high-resolution soot particle aerosol mass spectrometer data Z. Bibi et al. 10.5194/acp-21-10763-2021
- Combustion generated nanomaterials: online characterization via an ICP-MS based technique. Part II: resolving power for heterogeneous matrices D. Foppiano et al. 10.1039/C8JA00067K
- Chemical and physical characterization of traffic particles in four different highway environments in the Helsinki metropolitan area J. Enroth et al. 10.5194/acp-16-5497-2016
- Characterization of submicron aerosol chemical composition and sources in the coastal area of Central Chile S. Saarikoski et al. 10.1016/j.atmosenv.2018.11.040
- Review of black carbon emission factors from different anthropogenic sources T. Rönkkö et al. 10.1088/1748-9326/acbb1b
- Investigating the chemical species in submicron particles emitted by city buses S. Saarikoski et al. 10.1080/02786826.2016.1261992
- Comprehensive characterization of wintertime submicron aerosol in a Nordic town influenced by residential wood combustion, traffic and industrial sources L. Barreira et al. 10.1016/j.apr.2023.101835
- Trace Metals in Soot and PM2.5 from Heavy-Fuel-Oil Combustion in a Marine Engine J. Corbin et al. 10.1021/acs.est.8b01764
- Aerosol Measurements by Soot Particle Aerosol Mass Spectrometer: a Review Y. Zhang et al. 10.1007/s40726-020-00162-4
- Combustion generated nanomaterials: online characterization via an ICP-MS based technique. Part I: calibration strategy with a TGA D. Foppiano et al. 10.1039/C8JA00066B
- Laboratory and field evaluation of the Aerosol Dynamics Inc. concentrator (ADIc) for aerosol mass spectrometry S. Saarikoski et al. 10.5194/amt-12-3907-2019
- Production of N2O5 and ClNO2 through Nocturnal Processing of Biomass-Burning Aerosol A. Ahern et al. 10.1021/acs.est.7b04386
- Aqueous aging of secondary organic aerosol coating onto black carbon: Insights from simultaneous L-ToF-AMS and SP-AMS measurements at an urban site in southern China L. Cao et al. 10.1016/j.jclepro.2021.129888
- Household solid waste combustion with wood increases particulate trace metal and lung deposited surface area emissions H. Timonen et al. 10.1016/j.jenvman.2021.112793
- Characterizing metals in particulate pollution in communities at the fenceline of heavy industry: combining mobile monitoring and size-resolved filter measurements M. Tehrani et al. 10.1039/D3EM00142C
- Characterization of carbonaceous aerosols in Singapore: insight from black carbon fragments and trace metal ions detected by a soot particle aerosol mass spectrometer L. Rivellini et al. 10.5194/acp-20-5977-2020
- Effect of secondary organic aerosol coating thickness on the real-time detection and characterization of biomass-burning soot by two particle mass spectrometers A. Ahern et al. 10.5194/amt-9-6117-2016
- Sources, size-resolved deposition in the human respiratory tract and health risks of submicron black carbon in urban atmosphere in Pearl River Delta, China Y. Liu et al. 10.1016/j.scitotenv.2023.164391
- Atomic spectrometry update – a review of advances in environmental analysis O. Butler et al. 10.1039/C6JA90058E
- Online chemical characterization of atmospheric fine secondary aerosols and organic nitrates in summer Nanjing, China J. Xian et al. 10.1016/j.atmosres.2023.106783
- Chemical properties and single-particle mixing state of soot aerosol in Houston during the TRACER campaign R. Farley et al. 10.5194/acp-24-3953-2024
- Influence of fuel ethanol content on primary emissions and secondary aerosol formation potential for a modern flex-fuel gasoline vehicle H. Timonen et al. 10.5194/acp-17-5311-2017
- Distinguishing fuel and lubricating oil combustion products in diesel engine exhaust particles S. Carbone et al. 10.1080/02786826.2019.1584389
- Moving beyond Fine Particle Mass: High-Spatial Resolution Exposure to Source-Resolved Atmospheric Particle Number and Chemical Mixing State Q. Ye et al. 10.1289/EHP5311
- In-situ characterization of metal nanoparticles and their organic coatings using laser-vaporization aerosol mass spectrometry P. Nilsson et al. 10.1007/s12274-015-0877-9
25 citations as recorded by crossref.
- Influence of Emissions and Aqueous Processing on Particles Containing Black Carbon in a Polluted Urban Environment: Insights From a Soot Particle‐Aerosol Mass Spectrometer S. Collier et al. 10.1002/2017JD027851
- Technical note: A new approach to discriminate different black carbon sources by utilising fullerene and metals in positive matrix factorisation analysis of high-resolution soot particle aerosol mass spectrometer data Z. Bibi et al. 10.5194/acp-21-10763-2021
- Combustion generated nanomaterials: online characterization via an ICP-MS based technique. Part II: resolving power for heterogeneous matrices D. Foppiano et al. 10.1039/C8JA00067K
- Chemical and physical characterization of traffic particles in four different highway environments in the Helsinki metropolitan area J. Enroth et al. 10.5194/acp-16-5497-2016
- Characterization of submicron aerosol chemical composition and sources in the coastal area of Central Chile S. Saarikoski et al. 10.1016/j.atmosenv.2018.11.040
- Review of black carbon emission factors from different anthropogenic sources T. Rönkkö et al. 10.1088/1748-9326/acbb1b
- Investigating the chemical species in submicron particles emitted by city buses S. Saarikoski et al. 10.1080/02786826.2016.1261992
- Comprehensive characterization of wintertime submicron aerosol in a Nordic town influenced by residential wood combustion, traffic and industrial sources L. Barreira et al. 10.1016/j.apr.2023.101835
- Trace Metals in Soot and PM2.5 from Heavy-Fuel-Oil Combustion in a Marine Engine J. Corbin et al. 10.1021/acs.est.8b01764
- Aerosol Measurements by Soot Particle Aerosol Mass Spectrometer: a Review Y. Zhang et al. 10.1007/s40726-020-00162-4
- Combustion generated nanomaterials: online characterization via an ICP-MS based technique. Part I: calibration strategy with a TGA D. Foppiano et al. 10.1039/C8JA00066B
- Laboratory and field evaluation of the Aerosol Dynamics Inc. concentrator (ADIc) for aerosol mass spectrometry S. Saarikoski et al. 10.5194/amt-12-3907-2019
- Production of N2O5 and ClNO2 through Nocturnal Processing of Biomass-Burning Aerosol A. Ahern et al. 10.1021/acs.est.7b04386
- Aqueous aging of secondary organic aerosol coating onto black carbon: Insights from simultaneous L-ToF-AMS and SP-AMS measurements at an urban site in southern China L. Cao et al. 10.1016/j.jclepro.2021.129888
- Household solid waste combustion with wood increases particulate trace metal and lung deposited surface area emissions H. Timonen et al. 10.1016/j.jenvman.2021.112793
- Characterizing metals in particulate pollution in communities at the fenceline of heavy industry: combining mobile monitoring and size-resolved filter measurements M. Tehrani et al. 10.1039/D3EM00142C
- Characterization of carbonaceous aerosols in Singapore: insight from black carbon fragments and trace metal ions detected by a soot particle aerosol mass spectrometer L. Rivellini et al. 10.5194/acp-20-5977-2020
- Effect of secondary organic aerosol coating thickness on the real-time detection and characterization of biomass-burning soot by two particle mass spectrometers A. Ahern et al. 10.5194/amt-9-6117-2016
- Sources, size-resolved deposition in the human respiratory tract and health risks of submicron black carbon in urban atmosphere in Pearl River Delta, China Y. Liu et al. 10.1016/j.scitotenv.2023.164391
- Atomic spectrometry update – a review of advances in environmental analysis O. Butler et al. 10.1039/C6JA90058E
- Online chemical characterization of atmospheric fine secondary aerosols and organic nitrates in summer Nanjing, China J. Xian et al. 10.1016/j.atmosres.2023.106783
- Chemical properties and single-particle mixing state of soot aerosol in Houston during the TRACER campaign R. Farley et al. 10.5194/acp-24-3953-2024
- Influence of fuel ethanol content on primary emissions and secondary aerosol formation potential for a modern flex-fuel gasoline vehicle H. Timonen et al. 10.5194/acp-17-5311-2017
- Distinguishing fuel and lubricating oil combustion products in diesel engine exhaust particles S. Carbone et al. 10.1080/02786826.2019.1584389
- Moving beyond Fine Particle Mass: High-Spatial Resolution Exposure to Source-Resolved Atmospheric Particle Number and Chemical Mixing State Q. Ye et al. 10.1289/EHP5311
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Short summary
The purpose of this study was to develop a method for the quantification of trace metal content in black carbon aerosol in real time, such as combustion-related emissions, by using the SP-AMS. The properties of 13 different trace metals (Na, Al, Ca, V, Cr, Fe, Mn, Ni, Cu, Zn, Rb, Sr and Ba) were investigated in a controlled laboratory experiment. The results from the laboratory tests were applied to study fine particles in emissions of a heavy-fuel-oil-fired heating station.
The purpose of this study was to develop a method for the quantification of trace metal content...
