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Atmospheric Measurement Techniques An interactive open-access journal of the European Geosciences Union
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Volume 9, issue 3 | Copyright
Atmos. Meas. Tech., 9, 1063-1082, 2016
https://doi.org/10.5194/amt-9-1063-2016
© Author(s) 2016. This work is distributed under
the Creative Commons Attribution 3.0 License.

Research article 15 Mar 2016

Research article | 15 Mar 2016

New temperature and pressure retrieval algorithm for high-resolution infrared solar occultation spectroscopy: analysis and validation against ACE-FTS and COSMIC

Kevin S. Olsen1, Geoffrey C. Toon2, Chris D. Boone3, and Kimberly Strong1 Kevin S. Olsen et al.
  • 1Department of Physics, University of Toronto, Toronto, Ontario, Canada
  • 2Jet Propulsion Laboratory, California Institute of Technology, Pasadena, California, USA
  • 3Department of Chemistry, University of Waterloo, Waterloo, Ontario, Canada

Abstract. Motivated by the initial selection of a high-resolution solar occultation Fourier transform spectrometer (FTS) to fly to Mars on the ExoMars Trace Gas Orbiter, we have been developing algorithms for retrieving volume mixing ratio vertical profiles of trace gases, the primary component of which is a new algorithm and software for retrieving vertical profiles of temperature and pressure from the spectra. In contrast to Earth-observing instruments, which can rely on accurate meteorological models, a priori information, and spacecraft position, Mars retrievals require a method with minimal reliance on such data. The temperature and pressure retrieval algorithms developed for this work were evaluated using Earth-observing spectra from the Atmospheric Chemistry Experiment (ACE) FTS, a solar occultation instrument in orbit since 2003, and the basis for the instrument selected for a Mars mission. ACE-FTS makes multiple measurements during an occultation, separated in altitude by 1.5–5km, and we analyse 10 CO2 vibration–rotation bands at each altitude, each with a different usable altitude range. We describe the algorithms and present results of their application and their comparison to the ACE-FTS data products. The Constellation Observing System for Meteorology, Ionosphere, and Climate (COSMIC) provides vertical profiles of temperature up to 40km with high vertical resolution. Using six satellites and GPS radio occultation, COSMIC's data product has excellent temporal and spatial coverage, allowing us to find coincident measurements with ACE with very tight criteria: less than 1.5h and 150km. We present an intercomparison of temperature profiles retrieved from ACE-FTS using our algorithm, that of the ACE Science Team (v3.5), and from COSMIC. When our retrievals are compared to ACE-FTS v3.5, we find mean differences between −5 and +2K and that our retrieved profiles have no seasonal or zonal biases but do have a warm bias in the stratosphere and a cold bias in the mesosphere. When compared to COSMIC, we do not observe a warm/cool bias and mean differences are between −4 and +1K. COSMIC comparisons are restricted to below 40km, where our retrievals have the best agreement with ACE-FTS v3.5. When comparing ACE-FTS v3.5 to COSMIC we observe a cold bias in COSMIC of 0.5K, and mean differences are between −0.9 and +0.6K.

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A new version of the Atmospheric Chemistry Experiment Fourier transform spectrometer was intended to be sent to Mars to perform a detailed study of the composition of the Martian atmosphere. Of critical importance for such a mission is a method to accurately determine the temperature and pressure of the atmosphere. This paper presents a new algorithm for measuring temperature and pressure from high-resolution infrared spectra of CO2 absorption and applies it to terrestrial spectra.
A new version of the Atmospheric Chemistry Experiment Fourier transform spectrometer was...
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