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Volume 9, issue 3
Atmos. Meas. Tech., 9, 1095-1111, 2016
https://doi.org/10.5194/amt-9-1095-2016
© Author(s) 2016. This work is distributed under
the Creative Commons Attribution 3.0 License.
Atmos. Meas. Tech., 9, 1095-1111, 2016
https://doi.org/10.5194/amt-9-1095-2016
© Author(s) 2016. This work is distributed under
the Creative Commons Attribution 3.0 License.

Research article 18 Mar 2016

Research article | 18 Mar 2016

Global stratospheric measurements of the isotopologues of methane from the Atmospheric Chemistry Experiment Fourier transform spectrometer

Eric M. Buzan et al.
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Cited articles  
Allan, W., Manning, M. R., Lassey, K. R., Lowe, D. C., and Gomez, A. J.: Modeling the variation of δ13C in atmospheric methane: Phase ellipses and the kinetic isotope effect, Global Biogeochem. Cy., 15, 467–481, https://doi.org/10.1029/2000GB001282, 2001.
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Bartlett, K. B. and Harriss, R. C.: Review and assessment of methane emissions from wetlands, Chemosphere, 26, 261–320, https://doi.org/10.1016/0045-6535(93)90427-7, 1993.
Beale, C. A., Buzan, E. M., Boone, C. D., and Bernath, P. F.: Near-global distribution of CO isotopic fractionation in the Earth's atmosphere, J. Mol. Spectrosc., 1–8, https://doi.org/10.1016/j.jms.2015.12.005, 2015.
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This paper presents the first global data set of atmospheric concentrations of the isotopologues of methane as measured by ACE-FTS. Both CH3D and 13CH4 show enrichment at higher altitudes and some seasonal variation at the poles. After applying a constant correction factor to the CH3D data set, good agreement with existing balloon measurements is achieved. However, 13CH4 still shows a large amount of error. Improved lab measurements of CH4 would help reduce errors in the ACE-FTS data.
This paper presents the first global data set of atmospheric concentrations of the isotopologues...
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