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Atmospheric Measurement Techniques An interactive open-access journal of the European Geosciences Union
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Volume 9, issue 4
Atmos. Meas. Tech., 9, 1431–1447, 2016
https://doi.org/10.5194/amt-9-1431-2016
© Author(s) 2016. This work is distributed under
the Creative Commons Attribution 3.0 License.
Atmos. Meas. Tech., 9, 1431–1447, 2016
https://doi.org/10.5194/amt-9-1431-2016
© Author(s) 2016. This work is distributed under
the Creative Commons Attribution 3.0 License.

Research article 04 Apr 2016

Research article | 04 Apr 2016

Investigation of potential interferences in the detection of atmospheric ROx radicals by laser-induced fluorescence under dark conditions

Hendrik Fuchs et al.
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Ammann, M., Cox, R. A., Crowley, J. N., Jenkin, M. E., Mellouki, A., Rossi, M. J., Troe, J., and Wallington, T. J.: Evaluated kinetic and photochemical data for atmospheric chemistry: Volume VI – heterogeneous reactions with liquid substrates, Atmos. Chem. Phys., 13, 8045–8228, https://doi.org/10.5194/acp-13-8045-2013, 2013.
Aschmann, S. M., Arey, J., and Atkinson, R.: OH radical formation from the gas-phase reactions of O3 with a series of terpenes, Atmos. Environ., 36, 4347–4355, https://doi.org/10.1016/S1352-2310(02)00355-2, 2002.
Atkinson, R., Baulch, D. L., Cox, R. A., Crowley, J. N., Hampson, R. F., Hynes, R. G., Jenkin, M. E., Rossi, M. J., Troe, J., and IUPAC Subcommittee: Evaluated kinetic and photochemical data for atmospheric chemistry: Volume II – gas phase reactions of organic species, Atmos. Chem. Phys., 6, 3625–4055, https://doi.org/10.5194/acp-6-3625-2006, 2006.
Blitz, M. A., Heard, D. E., Pilling, M. J., Arnold, S. R., and Chipperfield, M. P.: Pressure and temperature-dependent quantum yields for the photodissociation of acetone between 279 and 327.5 nm, Geophys. Res. Lett., 31, L06111, https://doi.org/10.1029/2003GL018793, 2004.
Broch, S.: Ein neues LIF-Instrument für Flugzeug und Bodengebundene Messungen von OH und HO2 Radikalen in der Troposphäre, Thesis, 27–48, 2011.
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The hydroxyl radical is the key reactant that controls the chemical transformation of pollutants in the atmosphere. Observations of nighttime radicals concentrations were larger than predicted by models in field campaigns in forested and urban environments. Here, we investigated, if measurements could have been affected by artifacts. No significant interferences were found for atmospheric concentrations of reactants in ozonolysis experiments, but small artificats from nitrate radicals.
The hydroxyl radical is the key reactant that controls the chemical transformation of pollutants...
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