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Atmospheric Measurement Techniques An interactive open-access journal of the European Geosciences Union
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Volume 9, issue 4
Atmos. Meas. Tech., 9, 1871–1888, 2016
https://doi.org/10.5194/amt-9-1871-2016
© Author(s) 2016. This work is distributed under
the Creative Commons Attribution 3.0 License.
Atmos. Meas. Tech., 9, 1871–1888, 2016
https://doi.org/10.5194/amt-9-1871-2016
© Author(s) 2016. This work is distributed under
the Creative Commons Attribution 3.0 License.

Research article 28 Apr 2016

Research article | 28 Apr 2016

Retrieval of aerosol optical depth in the visible range with a Brewer spectrophotometer in Athens

Henri Diémoz1,2, Kostas Eleftheratos3,4, Stelios Kazadzis5, Vassilis Amiridis6, and Christos S. Zerefos4,7 Henri Diémoz et al.
  • 1ARPA Valle d'Aosta, Saint-Christophe, Italy
  • 2Institute of Atmospheric Science and Climate, CNR, Rome, Italy
  • 3Faculty of Geology and Geoenvironment, University of Athens, Athens, Greece
  • 4Biomedical Research Foundation, Academy of Athens, Athens, Greece
  • 5PMOD/WRC, Davos Dorf, Switzerland
  • 6National Observatory of Athens, Athens, Greece
  • 7Navarino Environmental Observatory, Messinia, Greece

Abstract. A MkIV Brewer spectrophotometer has been operating in Athens since 2004. Direct-sun measurements originally scheduled for nitrogen dioxide retrievals were reprocessed to provide aerosol optical depths (AODs) at a wavelength of about 440 nm. A novel retrieval algorithm was specifically developed and the resulting AODs were compared to those obtained from a collocated Cimel filter radiometer belonging to the Aerosol Robotic Network (AERONET). The series are perfectly correlated, with Pearson's correlation coefficients being as large as 0.996 and with 90 % of AOD deviations between the two instruments being within the World Meteorological Organisation (WMO) traceability limits. In order to reach such a high agreement, several instrumental factors impacting the quality of the Brewer retrievals must be taken into account, including sensitivity to the internal temperature, and the state of the external optics and pointing accuracy must be carefully checked. Furthermore, the long-term radiometric stability of the Brewer was investigated and the performances of in situ Langley extrapolations as a way to track the absolute calibration of the Brewer were assessed. Other sources of error, such as slight shifts of the wavelength scale, are discussed and some recommendations to Brewer operators are drawn. Although MkIV Brewers are rarely employed to retrieve AODs in the visible range, they represent a key source of information about aerosol changes in the past three decades and a potential worldwide network for present and future coordinated AOD measurements. Moreover, a better understanding of the AOD retrieval at visible wavelengths will also contribute in improving similar techniques in the more challenging UV range.

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Short summary
A new algorithm allowed to retrieve aerosol optical depths from a Brewer spectrophotometer in Athens with excellent agreement with AERONET. The instrument radiometric stability and the performances of in situ Langley extrapolations as a way to track it are investigated. Potential sources of error and recommendations to operators are reported. MkIV Brewers represent a great source of information about aerosols in the past decades and a promising worldwide network for coordinated AOD measurements.
A new algorithm allowed to retrieve aerosol optical depths from a Brewer spectrophotometer in...
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