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Atmospheric Measurement Techniques An interactive open-access journal of the European Geosciences Union

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Atmos. Meas. Tech., 9, 5089-5101, 2016
https://doi.org/10.5194/amt-9-5089-2016
© Author(s) 2016. This work is distributed under
the Creative Commons Attribution 3.0 License.
Research article
18 Oct 2016
MAX-DOAS retrieval of aerosol extinction properties in Madrid, Spain
Shanshan Wang1,a, Carlos A. Cuevas1, Udo Frieß2, and Alfonso Saiz-Lopez1 1Department of Atmospheric Chemistry and Climate, Institute of Physical Chemistry Rocasolano, CSIC, 28006 Madrid, Spain
2Institute of Environmental Physics, University of Heidelberg, 69120 Heidelberg, Germany
anow at: Shanghai Key Laboratory of Atmospheric Particle Pollution and Prevention (LAP), Department of Environmental Science & Engineering, Fudan University, 200433 Shanghai, China
Abstract. Multi-axis differential optical absorption spectroscopy (MAX-DOAS) measurements were performed in the urban environment of Madrid, Spain, from March to September 2015. The O4 absorption in the ultraviolet (UV) spectral region was used to retrieve the aerosol extinction profile using an inversion algorithm. The results show a good agreement between the hourly retrieved aerosol optical depth (AOD) and the correlative Aerosol Robotic Network (AERONET) product, with a correlation coefficient of R =  0.87. Higher AODs are found in the summer season due to the more frequent occurrence of Saharan dust intrusions. The surface aerosol extinction coefficient as retrieved by the MAX-DOAS measurements was also compared to in situ PM2.5 concentrations. The level of agreement between both measurements indicates that the MAX-DOAS retrieval has the ability to characterize the extinction of aerosol particles near the surface. The retrieval algorithm was also used to study a case of severe dust intrusion on 12 May 2015. The capability of the MAX-DOAS retrieval to recognize the dust event including an elevated particle layer is investigated along with air mass back-trajectory analysis.

Citation: Wang, S., Cuevas, C. A., Frieß, U., and Saiz-Lopez, A.: MAX-DOAS retrieval of aerosol extinction properties in Madrid, Spain, Atmos. Meas. Tech., 9, 5089-5101, https://doi.org/10.5194/amt-9-5089-2016, 2016.
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Short summary
Multi-axis differential optical absorption spectroscopy (MAX-DOAS) measurements were performed in the urban environment of Madrid, Spain, where Sahara dust intrusion sometimes occurs. The study shows a high performances in the retrieval of aerosol optical depth, the surface extinction coefficient and an elevated layer during dust episodes, validated by AERONET in situ and modeling data. It is essential to capture the extinction properties of both local aerosol and Saharan dust.
Multi-axis differential optical absorption spectroscopy (MAX-DOAS) measurements were performed...
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