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Atmospheric Measurement Techniques An interactive open-access journal of the European Geosciences Union
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Volume 9, issue 2 | Copyright
Atmos. Meas. Tech., 9, 721-740, 2016
https://doi.org/10.5194/amt-9-721-2016
© Author(s) 2016. This work is distributed under
the Creative Commons Attribution 3.0 License.

Research article 29 Feb 2016

Research article | 29 Feb 2016

Retrieval of near-surface sulfur dioxide (SO2) concentrations at a global scale using IASI satellite observations

Sophie Bauduin1, Lieven Clarisse1, Juliette Hadji-Lazaro2, Nicolas Theys3, Cathy Clerbaux1,2, and Pierre-François Coheur1 Sophie Bauduin et al.
  • 1Spectroscopie de l'atmosphère, Service de Chimie Quantique et Photophysique, Université Libre de Bruxelles (ULB), Brussels, Belgium
  • 2Sorbonne Universités, UPMC Univ. Paris 06, Université Versailles St-Quentin, CNRS/INSU, LATMOS-IPSL, Paris, France
  • 3Belgian Institute for Space Aeronomy (BIRA-IASB), Brussels, Belgium

Abstract. SO2 from volcanic eruptions is now operationally monitored from space in both the ultraviolet (UV) and thermal infrared (TIR) spectral range, but anthropogenic SO2 has almost solely been measured from UV sounders. Indeed, TIR instruments are well known to have a poor sensitivity to the planetary boundary layer (PBL), due to generally low thermal contrast (TC) between the ground and the air above it. Recent studies have demonstrated the capability of the Infrared Atmospheric Sounding Interferometer (IASI) to measure near-surface SO2 locally, for specific atmospheric conditions. In this work, we develop a retrieval method allowing the inference of SO2 near-surface concentrations from IASI measurements at a global scale. This method consists of two steps. Both are based on the computation of radiance indexes representing the strength of the SO2 ν3 band in IASI spectra. The first step allows the peak altitude of SO2 to be retrieved and near-surface SO2 to be selected. In the second step, 0–4km columns of SO2 are inferred using a look-up table (LUT) approach. Using this new retrieval method, we obtain the first global distribution of near-surface SO2 from IASI-A, and identify the dominant anthropogenic hotspot sources and volcanic degassing. The 7-year daily time evolution of SO2 columns above two industrial source areas (Beijing in China and Sar Cheshmeh in Iran) is investigated and correlated to the seasonal variations of the parameters that drive the IASI sensitivity to the PBL composition. Apart from TC, we show that humidity is the most important parameter which determines IR sensitivity to near-surface SO2 in the ν3 band. As IASI provides global measurements twice daily, the differences between the retrieved columns for the morning and evening orbits are investigated. This paper finally presents a first intercomparison of the measured 0–4km columns with an independent iterative retrieval method and with observations of the Ozone Monitoring Instrument (OMI).

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The paper presents the development of a new retrieval scheme to infer near-surface sulfur dioxide (SO2) concentrations at a global scale from the Infrared Atmospheric Sounding Interferometer (IASI). It demonstrates the capability of such an instrument to globally monitor anthropogenic SO2 pollution in the case of favourable geophysical conditions, especially high thermal contrast and low humidity.
The paper presents the development of a new retrieval scheme to infer near-surface sulfur...
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